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Discovery of Weyl semimetal state violating Lorentz invariance in MoTe2

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 نشر من قبل Nan Xu
 تاريخ النشر 2016
  مجال البحث فيزياء
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A new type of Weyl semimetal state, in which the energy values of Weyl nodes are not the local extrema, has been theoretically proposed recently, namely type II Weyl semimetal. Distinguished from type I semimetal (e.g. TaAs), the Fermi surfaces in a type II Weyl semimetal consist of a pair of electron and hole pockets touching at the Weyl node. In addition, Weyl fermions in type II Weyl semimetals violate Lorentz invariance. Due to these qualitative differences distinct spectroscopy and magnetotransport properties are expected in type II Weyl semimetals. Here, we present the direct observation of the Fermi arc states in MoTe2 by using angle resolved photoemission spectroscopy. Two arc states are identified for each pair of Weyl nodes whoes surface projections of them possess single topological charge, which is a unique property for type II Weyl semimetals. The experimentally determined Fermi arcs are consistent with our first principle calculations. Our results unambiguously establish that MoTe2 is a type II Weyl semimetal, which serves as a great test bed to investigate the phenomena of new type of Weyl fermions with Lorentz invariance violated.

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Topological quantum materials, including topological insulators and superconductors, Dirac semimetals and Weyl semimetals, have attracted much attention recently for their unique electronic structure, spin texture and physical properties. Very lately , a new type of Weyl semimetals has been proposed where the Weyl Fermions emerge at the boundary between electron and hole pockets in a new phase of matter, which is distinct from the standard type I Weyl semimetals with a point-like Fermi surface. The Weyl cone in this type II semimetals is strongly tilted and the related Fermi surface undergos a Lifshitz transition, giving rise to a new kind of chiral anomaly and other new physics. MoTe2 is proposed to be a candidate of a type II Weyl semimetal; the sensitivity of its topological state to lattice constants and correlation also makes it an ideal platform to explore possible topological phase transitions. By performing laser-based angle-resolved photoemission (ARPES) measurements with unprecedentedly high resolution, we have uncovered electronic evidence of type II semimetal state in MoTe2. We have established a full picture of the bulk electronic states and surface state for MoTe2 that are consistent with the band structure calculations. A single branch of surface state is identified that connects bulk hole pockets and bulk electron pockets. Detailed temperature-dependent ARPES measurements show high intensity spot-like features that is ~40 meV above the Fermi level and is close to the momentum space consistent with the theoretical expectation of the type II Weyl points. Our results constitute electronic evidence on the nature of the Weyl semimetal state that favors the presence of two sets of type II Weyl points in MoTe2.
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