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تسجيل مستخدم جديدMagnetostriction and magneto-structural domains in antiferromagnetic YBa$_{2}$Cu$_{3}$O$_{6}$
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We have used high-resolution neutron Larmor diffraction and capacitative dilatometry to investigate spontaneous and forced magnetostriction in undoped, antiferromagnetic YBa$_2$Cu$_3$O$_{6.0}$, the parent compound of a prominent family of high-temperature superconductors. Upon cooling below the Neel temperature, $T_N = 420$~K, Larmor diffraction reveals the formation of magneto-structural domains of characteristic size $sim 240$~nm. In the antiferromagnetic state, dilatometry reveals a minute ($4 times 10^{-6}$) orthorhombic distortion of the crystal lattice in external magnetic fields. We attribute these observations to exchange striction and spin-orbit coupling induced magnetostriction, respectively, and show that they have an important influence on the thermal and charge transport properties of undoped and lightly doped cuprates.
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We report results of a muon spin relaxation study of slow magnetic fluctuations in the pseudogap phase of underdoped single-crystalline YBa$_{2}$Cu$_{3}$O$_{y}$, $y = 6.77$ and 6.83. The dependence of the dynamic muon spin relaxation rate on applied
magnetic field yields the rms magnitude~$Bmathrm{_{loc}^{rms}}$ and correlation time~$tau_c$ of fluctuating local fields at muon sites. The observed relaxation rates do not decrease with decreasing temperature~$T$ below the pseudogap onset at $T^ast$, as would be expected for a conventional magnetic transition; both $Bmathrm{_{loc}^{rms}}$ and $tau_c$ are roughly constant in the pseudogap phase down to the superconducting transition. Corresponding NMR relaxation rates are estimated to be too small to be observable. Our results put strong constraints on theories of the anomalous pseudogap magnetism in YBa$_{2}$Cu$_{3}$O$_{y}$.
The present work addresses YBa$_{2}$Cu$_{3}$O$_{y}$ at doping below x=6% where the compound is a collinear antiferromagnet. In this region YBa$_{2}$Cu$_{3}$O$_{y}$ is a normal conductor with a finite resistivity at zero temperature. The value of the
staggered magnetization at zero temperature is 0.6mu_B, the maximum value allowed by spin quantum fluctuations. The staggered magnetization is almost independent of doping. On the other hand, the Neel temperature decays very quickly from T_N=420K at x=0 to practically zero at x = 0.06. The present paper explains these remarkable properties and demonstrates that the properties result from the physics of a lightly doped Mott insulator with small hole pockets. Nuclear quadrupole resonance data are also discussed. The data shed light on mechanisms of stability of the antiferromagnetic order at x < 6%.
Using neutron scattering, we investigate the effect of a magnetic field on the static and dynamic spin response in heavily underdoped superconducting YBa$_{2}$Cu$_{3}$O$_{6+x}$ (YBCO$_{6+x}$) with x=0.33 (T$_{c}$=8 K) and 0.35 (T$_{c}$=18 K). In cont
rast to the heavily doped and superconducting monolayer cuprates, the elastic central peak characterizing static spin correlations does not respond observably to a magnetic field which suppresses superconductivity. Instead, we find a magnetic field induced resonant enhancement of the spin fluctuations. The energy scale of the enhanced fluctuations matches the Zeeman energy within both the normal and vortex phases while the momentum dependence is the same as the zero field bilayer response. The magnitude of the enhancement is very similar in both phases with a fractional intensity change of $(I/I_{0}-1) sim 0.1$. We suggest that the enhancement is not directly correlated with superconductivity but is the result of almost free spins located near hole rich regions.
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