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The evolution of electron wavepackets determines the course of many physical and chemical phenomena and attosecond spectroscopy aims to measure and control such dynamics in real-time. Here, we investigate radial electron wavepacket motion in Helium by using an XUV attosecond pulse train to prepare a coherent superposition of excited states and a delayed femtosecond IR pulse to ionize them. Quantum beat signals observed in the high resolution photoelectron spectrogram allow us to follow the field-free evolution of the bound electron wavepacket and determine the time-dependent ionization dynamics of the low-lying 2p state.
Time-resolved pump-probe measurements of Xe, pumped at 133~nm and probed at 266~nm, are presented. The pump pulse prepared a long-lived hyperfine wavepacket, in the Xe $5p^5(^2P^{circ}_{1/2})6s~^2[1/2]^{circ}_1$ manifold ($E=$77185 cm$^{-1}=$9.57 eV)
We describe a numerical method that simulates the interaction of the helium atom with sequences of femtosecond and attosecond light pulses. The method, which is based on the close-coupling expansion of the electronic configuration space in a B-spline
X-ray four-wave mixing signals generated in the $k_1 + k_2 - k_3$ phase-matching direction are simulated for N1s transitions in para-nitroanline and two-ring hydrocarbons disubstituted with an amine and a nitroso groups. The two-dimensional x-ray cor
We report measurements of energy-dependent attosecond photoionization delays between the two outer-most valence shells of N$_2$O and H$_2$O. The combination of single-shot signal referencing with the use of different metal foils to filter the attosec
We study the role of electron-electron correlation in the ground-state of Ne, as well as in photoionization dynamics induced by an attosecond XUV pulse. For a selection of central photon energies around 100 eV, we find that while the mean-field time-