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Ott et al. (Science (340, 716 (2013)) successfully transferred Fano profile into Lorentzian lineshape using an intense infrared laser, after excitation of autoionizing states in helium by attosecond XUV pulse. This is a very important step forward of quantum phase control. However, here we show experimentally that an autoionizing state can have both Fano and Lorentzian behavior naturally, depending on the process involved. This study utilized the inverse process of photon absorption ionization, i.e. electron ion recombination with photon emission, making sure the resonant autoionizing state is not perturbed by the laser fields. Our result implies that excitation of the state through different paths can lead to different Fano profiles for the same resonant state. This allows more options for the combination of laser fields and lead to more opportunities for quantum phase control. Our result also indicates the breakdown of the classical two step picture for dielectronic recombination.
Multi-step laser resonance ionization spectroscopy of lutetium (Lu) has been performed at TRIUMFs off-line laser ion source test stand. The even-parity Rydberg series $6s^2nd$ $^2D_{3/2}$, $6s^2nd$ $^2D_{5/2}$ and $6s^2ns$ $^2S_{1/2}$ were observed c
We develop {it ab initio} relativistic QED theory for elastic electron scattering on hydrogen-like highly charged ions for impact energies where, in addition to direct (Coulomb) scattering, the process can also proceed via formation and consequent Au
Light-induced states are commonly observed in the photoionization spectra of laser-dressed atoms. The properties of autoionizing polaritons, entangled states of light and Auger resonances, however, are largely unexplored. We employ attosecond transie
Symmetric Lorentzian and asymmetric Fano line shapes are fundamental spectroscopic signatures that quantify the structural and dynamical properties of nuclei, atoms, molecules, and solids. This study introduces a universal temporal-phase formalism, m
Decay of bound states due to coupling with free particle states is a general phenomenon occurring at energy scales from MeV in nuclear physics to peV in ultracold atomic gases. Such a coupling gives rise to Fano-Feshbach resonances (FFR) that have be