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We have recently reported that the Haldane spin-chain system, Er2BaNiO5, undergoing antiferromagnetic order below 32 K, is characterized by the onset of ferroelectricity near 60K due to magnetoelectric coupling induced by short-range magnetic-order within spin-chains. We have carried out additional magnetic and dielectric studies to understand the properties well below antiferromagnetic ordering temperature. We emphasize here on the following: (i) A strong frequency dependent behaviors of ac magnetic susceptibility and complex dielectric properties have been observed at much lower temperatures (below 8 K), that is, reentrant multiglass-like phenomenon, naturally suggesting the existence of an additional transition well below Neel temperature; ii) Magnetoelectric phase coexistence is observed at very low temperature (e.g., T =2K), where the high-field magnetoelectric phase is partially arrested on returning to zero magnetic field after a cycling through metamagnetic transition.
The Haldane spin-chain (S=1) insulating compound, Sm2BaNiO5, which has been proposed to order antiferromagnetically around (T_N=) 55 K, was investigated for its complex dielectric permittivity, magnetodielectric and pyrocurrent behavior as a function
Static magnetic susceptibility chi, ac susceptibility chi_{ac} and specific heat C versus temperature T measurements on polycrystalline samples of In2VO5 and chi and C versus T measurements on the isostructural, nonmagnetic compound In2TiO5 are repor
We have investigated the magnetic behavior of the nano crystals, synthesized by high-energy ball-milling, for a well-known geometrically frustrated spin-chain system, Ca3CoRhO6, and compared its magnetic characteristics with those of the bulk form by
We report that the major features in the temperature dependence of dc and ac magnetization of a well-known spin-chain compound, Ca3Co2O6, which has been known to exhibit two complex magnetic transitions due to geometrical frustration (one near 24 K a
We have measured the specific heat of the S = 1/2 alternating Heisenberg antiferromagnetic chain compound pentafluorophenyl nitronyl nitroxide in magnetic fields using a single crystal and powder. A sharp peak due to field-induced magnetic ordering (