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We used polarization-dependent angle-resolved photoemission spectroscopy (ARPES) to study the high-energy anomaly (HEA) in the dispersion of Nd2-xCexCuO4, (x=0.123). We have found that at particular photon energies the anomalous, waterfalllike dispersion gives way to a broad, continuous band. This suggests that the HEA is a matrix element effect: it arises due to a suppression of the intensity of the broadened quasi-particle band in a narrow momentum range. We confirm this interpretation experimentally, by showing that the HEA appears when the matrix element is suppressed deliberately by changing the light polarization. Calculations of the matrix element using atomic wave functions and simulation of the ARPES intensity with one-step model calculations provide further proof for this scenario. The possibility to detect the full quasi-particle dispersion further allows us to extract the high-energy self-energy function near the center and at the edge of the Brillouin zone.
We analyse a model where the anomalies of the bond-stretching LO phonon mode are caused by the coupling to electron dynamic response in the form of a damped oscillator and explore the possibility to reconstruct the spectrum of the latter from the pho
The pursuit of a comprehensive understanding of the dynamical nature of intertwined orders in quantum matter has fueled the development of several new experimental techniques, including time- and angle-resolved photoemission spectroscopy (TR-ARPES).
Recently, angle-resolved photoemission spectroscopy has been used to highlight an anomalously large band renormalization at high binding energies in cuprate superconductors: the high energy waterfall or high energy anomaly (HEA). The anomaly is prese
High temperature superconductors have in common that they consist of parallel planes of copper oxide separated by layers whose composition can vary. Being ceramics, the cuprate superconductors are poor conductors above the transition temperature, T_c
On the basis of a semi-phenomenological model, it is argued that the high energy anomaly observed in recent photoemission experiments on cuprates is caused by interaction with an overdamped bosonic mode in the mid-infrared region of the spectrum. Ana