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Anisotropic rare-earth spin ensemble strongly coupled to a superconducting resonator

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 نشر من قبل Pavel Bushev
 تاريخ النشر 2012
  مجال البحث فيزياء
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Interfacing photonic and solid-state qubits within a hybrid quantum architecture offers a promising route towards large scale distributed quantum computing. Ideal candidates for coherent qubit interconversion are optically active spins magnetically coupled to a superconducting resonator. We report on a cavity QED experiment with magnetically anisotropic Er3+:Y2SiO5 crystals and demonstrate strong coupling of rare-earth spins to a lumped element resonator. In addition, the electron spin resonance and relaxation dynamics of the erbium spins are detected via direct microwave absorption, without aid of a cavity.

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Interfacing superconducting quantum processors, working in the GHz frequency range, with optical quantum networks and atomic qubits is a challenging task for the implementation of distributed quantum information processing as well as for quantum comm unication. Using spin ensembles of rare earth ions provide an excellent opportunity to bridge microwave and optical domains at the quantum level. In this letter, we demonstrate magnetic coupling of Er$^{3+}$ spins doped in Y$_{2}$SiO$_{5}$ crystal to a high-Q coplanar superconducting resonator.
We present cavity QED experiments with an Er:YSO crystal magnetically coupled to a 3D cylindrical sapphire loaded copper resonator. Such waveguide cavities are promising for the realization of a superconducting quantum processor. Here, we demonstrate the coherent integration of a rare-earth spin ensemble with the 3D architecture. The collective coupling strength of the Er$^{3+}$ spins to the 3D cavity is 21 MHz. The cylindrical sapphire loaded resonator allowed us to explore the anisotropic collective coupling between the rare-earth doped crystal and the cavity. This work shows the potential of spin doped solids in 3D quantum circuits for application as microwave quantum memories as well as for prospective microwave to optical interfaces.
We demonstrate the strong coupling between an electron spin ensemble and a three-dimensional cavity in a reflection geometry. We also find that an anticrossing in the cavity/spin spectrum can be observed under conditions that the collective coupling strength $g_c$ is smaller than the spin linewidth $gamma_s$ or the cavity linewidth. We identify a ratio of $g_c$ to $gamma_s$ ($g_c/gamma_s >$ 0.64) as a condition to observe a splitting in the cavity frequency. Finally, we confirm that $g_c$ scales with $sqrt{N}$, where $N$ is the number of polarized spins.
Yttrium orthosilicate (Y$_2$SiO$_5$, or YSO) has proved to be a convenient host for rare-earth ions used in demonstrations of microwave quantum memories and optical memories with microwave interfaces, and shows promise for coherent microwave--optical conversion owing to its favourable optical and spin properties. The strong coupling required by such microwave applications could be achieved using superconducting resonators patterned directly on Y$_2$SiO$_5$, and hence we investigate here the use of Y$_2$SiO$_5$ as an alternative to sapphire or silicon substrates for superconducting hybrid device fabrication. A NbN resonator with frequency 6.008 GHz and low power quality factor $Q approx 400000$ was fabricated on a Y$_2$SiO$_5$ substrate doped with isotopically enriched Nd$^{145}$. Measurements of dielectric loss yield a loss-tangent $tandelta = 4 times 10^{-6}$, comparable to sapphire. Electron spin resonance (ESR) measurements performed using the resonator show the characteristic angular dependence expected from the anisotropic Nd$^{145}$ spin, and the coupling strength between resonator and electron spins is in the high cooperativity regime ($C = 30$). These results demonstrate Y$_2$SiO$_5$ as an excellent substrate for low-loss, high-Q microwave resonators, especially in applications for coupling to optically-accessible rare earth spins.
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