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تسجيل مستخدم جديدMetastable Resistivity States and Conductivity Fluctuations in Low-doped La$_{1-x}$Ca$_{x}$MnO$_3$ Manganite Single Crystals
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Conductivity noise in dc current biased La_{0.82}Ca_{0.18}MnO_{3} single crystals has been investigated in different metastable resistivity states enforced by applying voltage pulses to the sample at low temperatures. Noise measured in all investigated resistivity states is of 1/f-type and its intensity at high temperatures and low dc bias scales as a square of the bias. At liquid nitrogen temperatures for under bias exceeding a threshold value, the behavior of the noise deviates from above quasi- equilibrium modulation noise and depends in a non monotonic way on applied bias. The bias range of nonequilibrium 1/f noise coincides with the range at which the conductance increases linearly with bias voltage. This feature is attributed to a broad continuity of states enabling indirect inelastic tunneling across intrinsic tunnel junctions. The nonequilibrium noise has been ascribed to indirect intrinsic tunneling mechanism while resistivity changes in metastable states to variations in the energy landscape for charge carriers introduced by microcracks created by the pulse procedures employed
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Low frequency noise in current biased La$_{0.82}$Ca$_{0.18}$MnO$_{3}$ single crystals has been investigated in a wide temperature range from 79 K to 290 K. Despite pronounced changes in magnetic properties and dissipation mechanisms of the sample wit
h changing temperature, the noise spectra were found to be always of the 1/f type and their intensity (except the lowest temperature studied) scaled as a square of the bias. At liquid nitrogen temperatures and under bias exceeding some threshold value, the behavior of the noise deviates from the quasi-equilibrium modulation noise and starts to depend in a non monotonic way on bias. It has been verified that the observed noise obeys Dutta and Horn model of 1/f noise in solids. The appearance of nonequilibrium 1/f noise and its dependence on bias have been associated with changes in the distribution of activation energies in the underlying energy landscape. These changes have been correlated with bias induced changes in the intrinsic tunneling mechanism dominating dissipation in La$_{0.82}$Ca$_{0.18}$MnO$_{3}$ at low temperatures.
Deterministic oscillations of current-induced metastable resistivity in changing voltage have been detected in La$_{0.82}$Ca$_{0.18}$MnO$_3$ single crystals. At low temperatures, below the Curie point, application of specific bias procedures switches
the crystal into metastable resistivity state characterized by appearance of pronounced reproducible and random structures in the voltage dependence of the differential conductivity. In certain bias range equally spaced broad conductivity peaks have been observed. The oscillating conductivity has been tentatively ascribed to resonances in a quantum well within the double tunnel barrier of intrinsic weak-links associated with twin-like defect boundaries.
We report new zero-field muon spin relaxation and neutron spin echo measurements in ferromagnetic (FM) (La,Ca)MnO3 which taken together suggest two spatially separated regions in close proximity possessing very different Mn-ion spin dynamics. One reg
ion corresponds to an extended cluster which displays critical slowing down near Tc and an increasing volume fraction below Tc. The second region possesses more slowly fluctuating spins and a decreasing volume fraction below Tc. These data are discussed in terms of the growth of small polarons into overlapping regions of correlated spins below Tc, resulting in a microscopically inhomogeneous FM transition.
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ated with charge ordering is found for all the samples. A magnetic field sufficient to induce the transition from the charge-ordered state to the ferromagnetic metallic state does not completely remove the $C^{prime}$ contribution. This suggests that the charge ordering is not completely destroyed by a melting magnetic field. In addition, the specific heat of the Pr$_{1-x}$Ca$_{x}$MnO$_{3}$ compounds exhibit a large contribution linear in temperature ($gamma T$) originating from magnetic and charge disorder.
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