اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدFerroelectric Soft Phonons, Charge Density Wave Instability and Strong Electron-Phonon Coupling in BiS2-Layered Superconductors
202
0
0.0
(
0
)
تأليف
Taner Yildirim
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
Very recently a new family of layered materials, containing BiS2 planes was discovered to be superconducting at temperatures up to Tc=10 K, raising questions about the mechanism of superconductivity in these systems. Here, we present state-of-the-art first principles calculations that directly address this question and reveal several surprising findings. The parent compound LaOBiS2 possesses anharmonic ferroelectric soft phonons at the zone center with a rather large polarization of $approx 10 mu C/cm^2$, which is comparable to the well-known ferroelectric BiFeO3. Upon electron doping, new unstable phonon branches appear along the entire line Q=(q,q,0), causing Bi/S atoms to order in a one-dimensional charge density wave (CDW). We find that BiS2 is a strong electron-phonon coupled superconductor in the vicinity of competing ferroelectric and CDW phases. Our results suggest new directions to tune the balance between these phases and increase Tc in this new class of materials.
قيم البحث
اقرأ أيضاً
The phonon-mode decomposition of the electron-phonon coupling in the MgB2-like system Li_{1-x}BC is explored using first principles calculations. It is found that the high temperature superconductivity of such systems results from extremely strong co
upling to only ~2% of the phonon modes. Novel characteristics of E_2g branches include (1) ``mode lambda values of 25 and greater compared to a mean of $sim 0.4$ for other modes, (2) a precipitous Kohn anomaly, and (3) E_2g phonon linewidths within a factor of ~2 of the frequency itself, indicating impending breakdown of linear electron-phonon theory. This behavior in borne out by recent inelastic x-ray scattering studies of MgB2 by Shukla et al.
Coupling between electrons and phonons (lattice vibrations) drives the formation of the electron pairs responsible for conventional superconductivity. The lack of direct evidence for electron-phonon coupling in the electron dynamics of the high trans
ition temperature superconductors has driven an intensive search for an alternative mechanism. A coupling of an electron with a phonon would result in an abrupt change of its velocity and scattering rate near the phonon energy. Here we use angle resolved photoemission spectroscopy to probe electron dynamics -velocity and scattering rate- for three different families of copper oxide superconductors. We see in all of these materials an abrupt change of electron velocity at 50-80meV, which we cannot explain by any known process other than to invoke coupling with the phonons associated with the movement of the oxygen atoms. This suggests that electron-phonon coupling strongly influences the electron dynamics in the high-temperature superconductors, and must therefore be included in any microscopic theory of superconductivity.
We present a combined density-functional-perturbation-theory and inelastic neutron scattering study of the lattice dynamical properties of YNi2B2C. In general, very good agreement was found between theory and experiment for both phonon energies and l
ine widths. Our analysis reveals that the strong coupling of certain low energy modes is linked to the presence of large displacements of the light atoms, i.e. B and C, which is unusual in view of the rather low phonon energies. Specific modes exhibiting a strong coupling to the electronic quasiparticles were investigated as a function of temperature. Their energies and line widths showed marked changes on cooling from room temperature to just above the superconducting transition at Tc = 15.2 K. Calculations simulating the effects of temperature allow to model the observed temperature dependence qualitatively.
The Kagome superconductors AV$_3$Sb$_5$ (A=K, Rb, Cs) have received enormous attention due to their nontrivial topological electronic structure, anomalous physical properties and superconductivity. Unconventional charge density wave (CDW) has been de
tected in AV$_3$Sb$_5$ that is found to be intimately intertwined with the anomalous Hall effect and superconductivity. High-precision electronic structure determination is essential to understand the origin of the CDW transition and its interplay with electron correlation, topology and superconductivity, yet, little evidence has been found about the impact of the CDW state on the electronic structure in AV$_3$Sb$_5$. Here we unveil electronic nature of the CDW phase in our high-resolution angle-resolved photoemission (ARPES) measurements on KV$_3$Sb$_5$. We have observed CDW-induced Fermi surface reconstruction and the associated band structure folding. The CDW-induced band splitting and the associated gap opening have been revealed at the boundary of the pristine and reconstructed Brillouin zone. The Fermi surface- and momentum-dependent CDW gap is measured for the first time and the strongly anisotropic CDW gap is observed for all the V-derived Fermi surface sheets. In particular, we have observed signatures of the electron-phonon coupling for all the V-derived bands. These results provide key insights in understanding the nature of the CDW state and its interplay with superconductivity in AV$_3$Sb$_5$ superconductors.
We study the effect of strong electron-phonon interactions on the damping of the Higgs amplitude mode in superconductors by means of non-equilibrium dynamical mean-field simulations of the Holstein model. In contrast to the BCS dynamics, we find that
the damping of the Higgs mode strongly depends on the temperature, becoming faster as the systen approaches the transition temperature. The damping at low temperatures is well described by a power-law, while near the transition temperature the damping shows exponential-like behavior. We explain this crossover by a temperature-dependent quasiparticle lifetime caused by the strong electron- phonon coupling, which smears the superconducting gap edge and makes the relaxation of the Higgs mode into quasiparticles more efficient at elevated temperatures. We also reveal that the phonon dynamics can soften the Higgs mode, which results in a slower damping.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
