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We calculate high-harmonic generation (HHG) by intense infrared lasers in atoms and molecules with the inclusion of macroscopic propagation of the harmonics in the gas medium. We show that the observed experimental spectra can be accurately reproduced theoretically despite that HHG spectra are sensitive to the experimental conditions. We further demonstrate that the simulated (or experimental) HHG spectra can be factored out as a product of a macroscopic wave packet and the photo-recombination transition dipole moment where the former depends on the laser properties and the experimental conditions, while the latter is the property of the target only. The factorization makes it possible to extract target structure from experimental HHG spectra, and for ultrafast dynamic imaging of transient molecules.
We study the effect of Coulomb potential on high-order harmonic generation (HHG) numerically and analytically. We focus on the influence of Coulomb potential on emission times of HHG associated with specific electron trajectories. By using a numerica
Using dynamical Hartree-Fock mean-field theory, we study the high-harmonic generation (HHG) in the fullerene molecules C$_{60}$ and C$_{70}$ under strong pump wave driving. We consider a strong-field regime and show that the output harmonic radiation
We report a study of high harmonic generation from noble gas clusters of xenon atoms in a gas jet. Harmonic spectra were investigated as a function of backing pressure, showing spectral shifts due to the nanoplasma electrons in the clusters. At certa
Recollision processes provide direct insight into the structure and dynamics of electronic wave functions. However, the strength of the process sets its basic limitations - the interaction couples numerous degrees of freedom. In this Letter we decoup
We investigate the role of excited states in High-order Harmonic Generation by studying the spectral, spatial and temporal characteristics of the radiation produced near the ionization threshold of argon by few-cycle laser pulses. We show that the po