اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدStructural Modification and Metamagnetic Anomaly in the Ordered State of CeOs2Al10
172
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
A caged compound CeOs2Al10, crystallizing in the orthorhombic YbFe2Al10-type structure, undergoes a mysterious phase transition at T_0=29 K. We report the results of electron diffraction, magnetization, and magnetoresistance for single crystals. Superlattice reflections characterized by a wave vector q = (0, -2/3, 2/3) observed at 15 K indicate a structural modification in the ordered state. Activation-type behavior of the electrical resistivity along the three principal axes below 50 K suggests gap opening in the conduction band. The magnetic susceptibility chi = M/B is highly anisotropic, chi_a>chi_c>chi_b, all of which sharply decrease on cooling below T_0. Furthermore, a metamagnetic anomaly in the magnetization and a step in the magnetoresistance occur at B=6-8 T only when the magnetic field is applied parallel to the orthorhombic c axis. However, T_0 hardly changes under magnetic fields up to 14 T, irrespective of the field direction. By using these data, we present a B-T phase diagram and discuss several scenarios for the mysterious transition.
قيم البحث
اقرأ أيضاً
The effect of Ir substitution for Os in CeOs2Al10, with an unusually high Neel temperature of T~28.5K, has been studied by high-resolution neutron diffraction and magnetization measurements. A small amount of Ir (~ 8%) results in a pronounced change
of the magnetic structure of the Ce-sublattice. The new magnetic ground state is controlled by the single ion anisotropy and implies antiferromagnetic arrangement of the Ce-moments along the a-axis, as expected from the anisotropy of the paramagnetic susceptibility. The value of the ordered moments, 0.92(1) mu_B, is substantially bigger than in the undoped compound, whereas the transition temperature is reduced down to 21K. A comparison of the observed phenomena with the recently studied CeRu1.9Rh0.1Al10 system, exhibiting similar behaviour [A. Kondo et al., J. Phys. Soc. Jpn. 82, 054709 (2013)], strongly suggests the electron doping as the main origin of the ground state changes. This provides a new way of exploring the anomalous magnetic properties of the Ce(Ru/Os)2Al10 compounds.
We have studied the magnetization of CeOs2Al10 in high magnetic fields up to 55 T for H // a and constructed the magnetic phase diagram for H // a. The magnetization curve shows a concave H dependence below T_max sim40 K which is higher than the tran
sition temperature T_0 sim29 K. The magnetic susceptibility along the a-axis shows a smooth and continuous decrease down to sim20 K below T_max sim40 K without showing an anomaly at T_0. From these two results, a Kondo singlet is formed below T_max and coexists with the antiferro magnetic order below T_0. We also propose that the larger suppression of the spin degrees of freedom along the a-axis than along the c-axis below T_max is associated with the origin of the antiferro magnetic component.
We investigated the effect of pressure on the magnetic and thermoelectric properties of Sr$_{3.1}$Y$_{0.9}$Co$_{4}$O$_{10+delta }$. The magnetization is reduced with the application of pressure, reflecting the spin-state modification of the Co$^{3+}$
ions into the nonmagnetic low-spin state. Accordingly, with increasing pressure, the Seebeck coefficient is enhanced, especially at low temperatures, at which the effect of pressure on the spin state becomes significant. These results indicate that the spin-orbital entropy is a key valuable for the thermoelectric properties of the strongly correlated cobalt oxides.
PrV$_2$Al$_{20}$ is a rare example of a heavy fermion system based on strong hybridization between conduction electrons and nonmagnetic quadrupolar moments of the cubic $Gamma_3$ ground doublet. Here, we report that a high-quality single crystal of P
rV$_2$Al$_{20}$ exhibits superconductivity at $T_{rm c}=$ 50 mK in the antiferroquadrupole-ordered state under ambient pressure. The heavy fermion character of the superconductivity is evident from the specific heat jump of $Delta C/T sim 0.3$ J/mol K$^2$ and the effective mass $m^*/m_0 sim 140$ estimated from the temperature dependence of the upper critical field. Furthermore, the high-quality single crystals exhibit double transitions at $T_{rm Q}$ = 0.75 K and $T^{*}$ = 0.65 K associated with quadrupole and octapole degrees of freedom of the $Gamma_3$ doublet. In the ordered state, the specific heat $C/T$ shows a $T^3$ dependence, indicating the gapless mode associated with the quadrupole and/or octapole order. The strong sensitivity to impurity of the superconductivity suggests unconventional character due to significant quadrupolar fluctuations.
Based on the four-band continuum model, we study the ordered-current state (OCS) for electrons in bilayer graphene at the charge neutrality point. The present work resolves the puzzles that (a) the energy gap increases significantly with increasing t
he magnetic field $B$, (b) the energy gap can be closed by the external electric field of either polarization, and (c) the particle-hole spectrum is asymmetric in the presence of $B$, all these as observed by the experiment. We also present the prediction of the hysteresis energy gap behavior with varying $B$, which explains the existing experimental observation on the electric conductance at weak $B$. The large energy gap of the OCS is shown to originate from the disappearance of Landau levels of $n$ = 0 and 1 states in conduction/valence band. By comparing with the existing models and the experiments, we conclude that the OCS is a possible ground state of electrons in bilayer graphene.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
