ترغب بنشر مسار تعليمي؟ اضغط هنا

Crystal orientation and thickness dependence of superconductivity on tetragonal FeSe1-x thin films

141   0   0.0 ( 0 )
 نشر من قبل Ming-Jye Wang
 تاريخ النشر 2009
  مجال البحث فيزياء
والبحث باللغة English
 تأليف M.J. Wang




اسأل ChatGPT حول البحث

Superconductivity was recently found in the simple tetragonal FeSe structure. Recent studies suggest that FeSe is unconventional, with the symmetry of the superconducting pairing state still under debate. To tackle these problems, clean single crystals and thin films are required. Here we report the fabrication of superconducting beta-phase FeSe1-x thin films on different substrates using a pulsed laser deposition (PLD) technique. Quite interestingly, the crystal orientation, and thus, superconductivity in these thin films is sensitive to the growth temperature. At 320C, films grow preferably along c-axis, but the onset of superconductivity depends on film thickness. At 500C, films grow along (101), with little thickness dependence. These results suggest that the low temperature structural deformation previously found is crucial to the superconductivity of this material.

قيم البحث

اقرأ أيضاً

80 - B. X. Wu , K. Jin , J. Yuan 2009
A series of electron-doped cuprate La(2-x)CexCuO4 thin films with different thicknesses have been fabricated and their annealing time are adjusted carefully to ensure the highest superconducting transition temperature. The transport measurements indi cate that, with the increase of the film thickness (<100 nm), the residual resistivity increases and the Hall coefficient shifts in the negative direction. Further more, the X-ray diffraction data reveal that the c-axis lattice constant c0 increases with the decrease of film thickness. These abnormal phenomena can be attributed to the insufficient oxygen reduction in the thin films. Considering the lattice mismatching in the ab-plane between the SrTiO3 substrates and the films, the compressive stress from the substrates may be responsible for the more difficult reduction of the oxygen in the thin films.
Due to competing long range ferromagnetic order, the transition metals Fe, Co and Ni are not superconductors at ambient pressure. While superconductivity was observed in a non-magnetic phase of Fe, stabilized under pressure, it is yet to be discovere d in Co and Ni under any experimental conditions. Here, we report emergence of superconductivity in the recently discovered high-density nonmagnetic face centered cubic phase in Co thin films below a transition temperature (Tc) of ~5.4 K, as revealed in experiments based on point-contact spectroscopy and resistance, and four-probe measurements of resistance at ambient pressure. We confirm the non-magnetic nature of the dense fcc phase of Co within first-principles density functional theory, and show that its superconductivity below 5 K originates from anomalous softening of zone-boundary phonons and their enhanced coupling with electrons upon biaxial strain.
We have studied the effect of deposition rate and layer thickness on the properties of epitaxial MgB2 thin films grown by hybrid physical-chemical vapor deposition on 4H-SiC substrates. The MgB2 film deposition rate depends linearly on the concentrat ion of B2H6 in the inlet gas mixture. We found that the superconducting and normal-state properties of the MgB2 films are determined by the film thickness, not by the deposition rate. When the film thickness was increased, the transition temperature, Tc, increased and the residual resistivity, rho0, decreased. Above about 300 nm, a Tc of 41.8 K, a rho0 of 0.28 mikroOhm.cm, and a residual resistance ratio RRR of over 30 were obtained. These values represent the best MgB2 properties reported thus far.
Among the magnetostrictive alloys the one formed of iron and gallium (called Galfenol from its U.S. Office of Naval Research discoverers in the late 90s) is attractive for its low hysteresis, good tensile stress, good machinability and its rare-earth free composition. One of its applications is its association with a piezoelectric material to form a extrinsic multiferroic composite as an alternative to the rare room temperature intrinsic multiferroics such as BiFeO$_3$. This study focuses on thin Fe$_{0.81}$Ga$_{0.19}$ films of thickness 5, 10, 20 and 60 nm deposited by sputtering onto glass substrates. Magnetization reversal study reveals a well-defined symmetry with two principal directions independent of the thickness. The magnetic signature of this magnetic anisotropy decreases with increasing FeGa thickness due to an increase of the non-preferential polycrystalline arrangement, as revealed by transmission electron microscopy (TEM) observations. Thus when magnetic field is applied along these specific directions, magnetization reversal is mainly coherent for the thinnest sample as seen from the transverse magnetization cycles. Magnetostriction coefficient reaches 20 ppm for the 5 nm film and decreases for thicker samples, where polycrystalline part with non-preferential orientation prevails.
We have successfully observed quantum oscillation (QO) for FeTe_{1-x}Se_{x}. QO measurements were performed using non-superconducting and superconducting thin crystals of FeTe_{0.65}Se_{0.35} fabricated by the scotch-tape method. We show that the Fer mi surfaces (FS) of the non-superconducting crystal are in good agreement with the rigid band shift model based on electron doping by excess Fe while that of the superconducting crystal is in good agreement with the calculated FS with no shift. From the FS comparison of both crystals, we demonstrate the change of the cross-sectional area of the FS, suggesting that the suppression of the FS nesting with the vector Q_{s} = (pi, pi) due to excess Fe results in the disappearance of the superconductivity.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا