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Ultralow-field nuclear magnetic resonance (NMR) provides a new regime for many applications ranging from materials science to fundamental physics. However, the experimentally observed spectra show asymmetric amplitudes, differing greatly from those predicted by the standard theory. Its physical origin remains unclear, as well as how to suppress it. Here we provide a comprehensive model to explain the asymmetric spectral amplitudes, further observe more unprecedented asymmetric spectroscopy and find a way to eliminate it. Moreover, contrary to the traditional idea that asymmetric phenomena were considered as a nuisance, we show that more information can be gained from the asymmetric spectroscopy, e.g., the light shift of atomic vapors and the sign of Land$acute{textrm{e}}$ $g$ factor of NMR systems.
As a complementary analysis tool to conventional high-field NMR, zero- to ultralow-field (ZULF) NMR detects nuclear magnetization signals in the sub-microtesla regime. Spin-exchange relaxation-free (SERF) atomic magnetometers provide a new generation
Zero- to ultralow-field nuclear magnetic resonance (ZULF NMR) is an alternative spectroscopic method to high-field NMR, in which samples are studied in the absence of a large magnetic field. Unfortunately, there is a large barrier to entry for many g
The nature of dark matter, the invisible substance making up over $80%$ of the matter in the Universe, is one of the most fundamental mysteries of modern physics. Ultralight bosons such as axions, axion-like particles or dark photons could make up mo
Nuclear magnetic resonance (NMR) spectroscopy has approached the limit of single molecule sensitivity, however the spectral resolution is currently insufficient to obtain detailed information on chemical structure and molecular interactions. Here we
This paper describes a general method for manipulation of nuclear spins in zero magnetic field. In the absence of magnetic fields, the spins lose the individual information on chemical shifts and inequivalent spins can only be distinguished by nuclea