ترغب بنشر مسار تعليمي؟ اضغط هنا

Replicas of the Kondo peak due to electron-vibration interaction in molecular transport properties

78   0   0.0 ( 0 )
 نشر من قبل Pablo Roura-Bas Dr.
 تاريخ النشر 2016
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

The low temperature properties of single level molecular quantum dots including both, electron-electron and electron-vibration interactions, are theoretically investigated. The calculated differential conductance in the Kondo regime exhibits not only the zero bias anomaly but also side peaks located at bias voltages which coincide with multiples of the energy of vibronic mode $V sim hbarOmega/e$. We obtain that the evolution with temperature of the two main satellite conductance peaks follows the corresponding one of the Kondo peak when $hbarOmega gg k_B T_K$, being $ T_K$ the Kondo temperature, in agreement with recent transport measurements in molecular junctions. However, we find that this is no longer valid when $ hbarOmega$ is of the order of a few times $k_B T_K$.



قيم البحث

اقرأ أيضاً

117 - P. Roura-Bas , F. Guller , L. Tosi 2019
We study the transport through a molecular junction exhibiting interference effects. We show that these effects can still be observed in the presence of molecular vibrations if Coulomb repulsion is taken into account. In the Kondo regime, the conduct ance of the junction can be changed by several orders of magnitude by tuning the levels of the molecule, or displacing a contact between two atoms, from nearly perfect destructive interference to values of the order of 2e 2 /h expected in Kondo systems. We also show that this large conductance change is robust for reasonable temperatures and voltages for symmetric and asymmetric tunnel couplings between the source-drain electrodes and the molecular orbitals. This is relevant for the development of quantum interference effect transistors based on molecular junctions.
We consider the Kondo effect arising from a hydrogen impurity in graphene. As a first approximation, the strong covalent bond to a carbon atom removes that carbon atom without breaking the $C_{3}$ rotation symmetry, and we only retain the Hubbard int eraction on the three nearest neighbors of the removed carbon atom which then behave as magnetic impurities. These three impurity spins are coupled to three conduction channels with definite helicity, two of which support a diverging local density of states (LDOS) $propto 1/ [ | omega | ln ^{2}( Lambda /| omega | ) ] $ near the Dirac point $omega rightarrow 0$ even though the bulk density of states vanishes linearly. We study the resulting 3-impurity multi-channel Kondo model using the numerical renormalization group method. For weak potential scattering, the ground state of the Kondo model is a particle-hole symmetric spin-$1/2$ doublet, with ferromagnetic coupling between the three impurity spins; for moderate potential scattering, the ground state becomes a particle-hole asymmetric spin singlet, with antiferromagnetic coupling between the three impurity spins. This behavior is inherited by the Anderson model containing the hydrogen impurity and all four carbon atoms in its vicinity.
142 - B. Y. Pan , H. C. Xu , Y. Liu 2020
CrAs is a well-known helimagnet with the double-helix structure originating from the competition between the Dzyaloshinskii-Moriya interaction (DMI) and antiferromagnetic exchange interaction $J$. By resonant soft X-ray scattering (RSXS), we observe the magnetic peak (0~0~$q_m$) that emerges at the helical transition with $T_S$ $approx$ 267.5 K. Intriguingly, the helimagnetic domains significantly shrink on cooling below $sim$255 K, opposite to the conventional thermal effect. The weakening of DMI on cooling is found to play a critical role here. It causes the helical wave vector to vary, ordered spins to rotate, and extra helimagnetic domain boundaries to form at local defects, thus leading to the anomalous shrinkage of helimagnetic domains. Our results indicate that the size of magnetic helical domains can be controlled by tuning DMI in certain helimagnets.
The authors report micro-Raman investigation of changes in the single and bilayer graphene crystal lattice induced by the low and medium energy electron-beam irradiation (5 and 20 keV). It was found that the radiation exposures results in appearance of the strong disorder D band around 1345 1/cm indicating damage to the lattice. The D and G peak evolution with the increasing radiation dose follows the amorphization trajectory, which suggests graphenes transformation to the nanocrystalline, and then to amorphous form. The results have important implications for graphene characterization and device fabrication, which rely on the electron microscopy and focused ion beam processing.
We address the optical conductivity of undoped bilayer graphene in the presence of a finite bias voltage at finite temperature. The effects of gap parameter and stacking type on optical conductivity are discussed in the context of tight binding model Hamiltonian. Greens function approach has been implemented to find the behavior of optical conductivity of bilayer graphene within linear response theory. We have found the frequency dependence of optical conductivity for different values of gap parameter and bias voltage. Also the dependence of optical conductivity on the temperature has been investigated in details. A peak appears in the plot of optical conductivity versus frequency for different values of temperatures and bias voltage. Furthermore we find the frequency position of broad peak in optical conductivity goes to higher values with increase of gap parameter for both bernal and simple stacked bilayer graphenes.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا