We report the systematic studies of spin current transport and relaxation mechanism in highly doped organic polymer film. In this study, we have determined spin diffusion length (SDL), spin lifetime, and spin diffusion constant by using different exp
erimental techniques. The spin lifetime estimated from the electron paramagnetic resonance experiment is much shorter than the previous expectation beyond the experimental ambiguity. This suggests that significantly large spin diffusion constant, which is reasonably explained by the hopping transport mechanism in degenerate semiconductors, exists in highly doped organic semiconductors. The calculated SDL using the spin lifetime and spin diffusion constant estimated from our experiment is comparable to the experimentally obtained SDL of the order of one hundred nanometers. Moreover, the present study revealed that the spin angular momentum is almost preserved in the hopping events. In other words, the spin relaxation mainly occurs due to the spin-orbit coupling at the nanoscale crystalline grains.
Cyclotron resonance (CR) measurements for the Fe-based superconductor KFe$_2$As$_2$ are performed. One signal for CR is observed, and is attributed to the two-dimensional $alpha$ Fermi surface at the $Gamma$ point. We found a large discrepancy in the
effective masses of CR [(3.4$pm$0.05)$m_e$ ($m_e$ is the free electron mass)] and de-Haas van Alphen (dHvA) results, a direct evidence of mass enhancement due to electronic correlation. A comparison of the CR and dHvA results shows that both intra- and interband electronic correlations contribute to the mass enhancement in KFe$_2$As$_2$.
We report the results of the angular-dependent magnetoresistance oscillations (AMROs), which can determine the shape of bulk Fermi surfaces in quasi-two-dimensional (Q2D) systems, in a highly hole-doped Fe-based superconductor KFe$_2$As$_2$ with $T_c
approx$ 3.7 K. From the AMROs, we determined the two Q2D FSs with rounded-square cross sections, corresponding to 12% and 17% of the first Brillouin zone. The rounded-squared shape of the FS cross section is also confirmed by the analyses of the interlayer transport under in-plane fields. From the obtained FS shape, we infer the character of the 3d orbitals that contribute to the FSs.
