Imaging an aligned polyatomic molecule with laser-induced electron diffraction

Laser-induced electron diffraction is an evolving tabletop method, which aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-{AA}ngstrom spatial and femtosecond temporal resolution. Here, we provide the general foundation for the retrieval of multiple bond lengths from a polyatomic molecule by simultaneously measuring the C-C and C-H bond lengths in aligned acetylene. Our approach takes the method beyond the hitherto achieved imaging of simple diatomic molecules and is based upon the combination of a 160 kHz mid-IR few-cycle laser source with full three-dimensional electron-ion coincidence detection. Our technique provides an accessible and robust route towards imaging ultrafast processes in complex gas phase molecules with atto- to femto-second temporal resolution.

Efficient generation of >2 W of green light by single pass frequency doubling in PPMgLN

We report 32% efficient frequency doubling of single frequency 1029 nm light to green light at 514.5 nm using a single pass configuration. A congruent composition, periodically poled magnesium doped lithium niobate (PPMgLN) crystal of 50 mm length was used to generate a second harmonic power of 2.3 W. To our knowledge, this is the highest reported frequency doubling efficiency of any wavelength light in a PPMgLN crystal and also the highest reported SHG output power in the green for PPMgLN.