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We experimentally study the spin dynamics of mesoscopic ensembles of ultracold magnetic spin-3 atoms located in two separated wells of an optical dipole trap. We use a radio-frequency sweep to selectively flip the spin of the atoms in one of the well s, which produces two separated spin domains of opposite polarization. We observe that these engineered spin domains are metastable with respect to the long-range magnetic dipolar interactions between the two ensembles. The absence of inter-cloud dipolar spin-exchange processes reveals a classical behavior, in contrast to previous results with atoms loaded in an optical lattice. When we merge the two subsystems, we observe spin-exchange dynamics due to contact interactions which enable the first determination of the s-wave scattering length of 52Cr atoms in the S=0 molecular channel a_0=13.5^{+11}_{-10.5}a_B (where a_B is the Bohr radius).
We study dipolar relaxation of a chromium BEC loaded into a 3D optical lattice. We observe dipolar relaxation resonances when the magnetic energy released during the inelastic collision matches an excitation towards higher energy bands. A spectroscop y of these resonances for two orientations of the magnetic field provides a 3D band spectroscopy of the lattice. The narrowest resonance is registered for the lowest excitation energy. Its line-shape is sensitive to the on-site interaction energy. We use such sensitivity to probe number squeezing in a Mott insulator, and we reveal the production of three-body states with entangled spin and orbital degrees of freedom.
We measure the excitation spectrum of a dipolar Chromium Bose Einstein Condensate with Raman-Bragg spectroscopy. The energy spectrum depends on the orientation of the dipoles with respect to the excitation momentum, demonstrating an anisotropy which originates from the dipole-dipole interactions between the atoms. We compare our results with the Bogoliubov theory based on the local density approximation, and, at large excitation wavelengths, with numerical simulations of the time dependent Gross-Pitaevskii equation. Our results show an anisotropy of the speed of sound
We observe interband transitions mediated by the dipole-dipole interaction for an array of 1D quantum gases of chromium atoms, trapped in a 2D optical lattice. Interband transitions occur when dipolar relaxation releases an energy which matches or ov ercomes the lattice band gap. We analyze the role of tunneling in higher lattice bands on this process. We compare the experimental dipolar relaxation rate with a calculation based on a multiple Fermi Golden Rule approach, when the lattice sites are symmetric, and the magnetic field is parallel to the lattice axis. We also show that an almost complete suppression of dipolar relaxation is obtained below a magnetic field threshold set by the depth of the lattice: 1D quantum gases in an excited Zeeman state then become metastable.
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