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116 - K. Iida , S.-H. Lee , T. Onimaru 2012
Magnetic excitations in a Ni$_4$ magnetic molecule were investigated by inelastic neutron scattering and bulk susceptibility ($chi_text{bulk}$) techniques. The magnetic excitation spectrum obtained from the inelastic neutron scattering experiments ex hibits three modes at energy transfers of $hbaromega=0.5$, 1.35, and 1.6 meV. We show that the energy, momentum, and temperature dependences of the inelastic neutron scattering data and $chi_text{bulk}$ can be well reproduced by an effective spin Hamiltonian consisted of intra-molecule exchange interactions, a single-ionic anisotropy, biquadratic interactions, and Zeeman term. Under a hydrostatic pressure, the bulk magnetization decreases with increasing pressure, which along with the biquadratic term indicates spin-lattice coupling present in this system.
366 - K. Iida , J. Lee , M. B. Stone 2012
We investigate the imaginary part of the wave vector dependent dynamic spin susceptibility in Sr$_2$(Ru$_{0.99}$Ti$_{0.01}$)O$_4$ as a function of temperature using neutron scattering. At T=5 K, two-dimensional incommensurate (IC) magnetic fluctuatio ns are clearly observed around $mathbf{Q}_text{c}=(0.3,0.3,L)$ up to approximately 60 meV energy transfer. We find that the IC excitations disperse to ridges around the $(pi,pi)$ point. Below 50 K, the energy and temperature dependent excitations are well described by the phenomenological response function for a Fermi liquid system with a characteristic energy of 4.0(1) meV. Although the wave vector dependence of the IC magnetic fluctuations in Sr$_2$(Ru$_{0.99}$Ti$_{0.01}$)O$_4$ is similar to that in the Fermi liquid state of the parent compound, Sr$_2$RuO$_4$, the magnetic fluctuations are clearly suppressed by the Ti-doping.
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