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Studies to date on ferromagnet/d-wave superconductor heterostructures focus mainly on the effects at or near the interfaces while the response of bulk properties to heterostructuring is overlooked. Here we use resonant soft x-ray scattering spectrosc opy to reveal a novel c-axis ferromagnetic coupling between the in-plane Cu spins in YBa$_2$ Cu$_3$ O$_{7-x}$ (YBCO) superconductor when it is grown on top of ferromagnetic La$_{0.7}$ Ca$_{0.3}$ MnO$_3$ (LCMO) manganite layer. This coupling, present in both normal and superconducting states of YBCO, is sensitive to the interfacial termination such that it is only observed in bilayers with MnO_2but not with La$_{0.7}$ Ca$_{0.3}$ interfacial termination. Such contrasting behaviors, we propose, are due to distinct energetic of CuO chain and CuO$_2$ plane at the La$_{0.7}$ Ca$_{0.3}$ and MnO$_2$ terminated interfaces respectively, therefore influencing the transfer of spin-polarized electrons from manganite to cuprate differently. Our findings suggest that the superconducting/ferromagnetic bilayers with proper interfacial engineering can be good candidates for searching the theorized Fulde-Ferrel-Larkin-Ovchinnikov (FFLO) state in cuprates and studying the competing quantum orders in highly correlated electron systems.
The total spectral weight textit{S} of the emergent low-energy quasipaticles in high-temperature superconductors is explored by x-ray absorption spectroscopy. In order to examine the applicability of the Hubbard model, regimes that cover from zero do ping to overdoping are investigated. In contrast to mean field theory, we found that textit{S} deviates from linear dependence on the doping level textit{p}. The slope of textit{S} versus textit{p} changes continuously throughout the whole doping range with no sign of saturation up to textit{p} = 0.23. Therefore, the picture of Zhang-Rice singlet remains intact within the most prominent doping regimes of HTSCs.
305 - C. W. Luo , C. C. Lee , H.-J. Chen 2013
This study shows that a terahertz (THz) wave can be generated from the (001) surface of cleaved Bi$_{textrm{2}}$Se$_{textrm{3}}$ and Cu-doped Bi$_{textrm{2}}$Se$_{textrm{3}}$ single crystals using 800 nm femtosecond pulses. The generated THz power is strongly dependent on the carrier concentration of the crystals. An examination of the dependence reveals the two-channel free carrier absorption to which Dirac fermions are indispensable. Dirac fermions in Bi$_{textrm{2}}$Se$_{textrm{3}}$ are significantly better absorbers of THz radiation than bulk carriers at room temperature. Moreover, the characteristics of THz emission confirm the existence of a recently proposed surface phonon branch that is normalized by Dirac fermions.
155 - C. W. Luo , I. H. Wu , P. C. Cheng 2012
Quasiparticle dynamics of FeSe single crystals revealed by dual-color transient reflectivity measurements ({Delta}R/R) provides unprecedented information on Fe-based superconductors. The amplitude of fast component in {Delta}R/R clearly tells a compe ting scenario between spin fluctuations and superconductivity. Together with the transport measurements, the relaxation time analysis further exhibits anomalous changes at 90 K and 230 K. The former manifests a structure phase transition as well as the associated phonon softening. The latter suggests a previously overlooked phase transition or crossover in FeSe. The electron-phonon coupling constant {lambda} is found to be 0.16, identical to the value of theoretical calculations. Such a small {lambda} demonstrates an unconventional origin of superconductivity in FeSe.
120 - J.-Y. Lin , P. R. Lee , Y. T. Liu 2010
The comprehensive study of the temperature dependent x-ray absorption spectroscopy (XAS) reveals a dynamical spectral weight $alpha$ in YBa$_2$Cu$_3$O$_y$ (YBCO). Large spectral weight changes for both the Upper Hubbard band and the Zhang-Rice band d ue to dynamics of holes are experimentally found in the underdoped regime. A large value of $alpha geq 0.3$ is indispensable to describing XAS of YBCO with the conservation of states. The value of $alpha$ is linearly proportional to the pseudogap temperature in the underdoped regime, but becomes smaller as the doping level goes to the undoped limit. Our results clearly indicate that the pseudogap is related to the double occupancy and originates from bands in higher energies.
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