We demonstrate the sensitivity of transverse-field muon spin rotation (TF-muSR) to static charge-density-wave (CDW) order in the bulk of 2H-NbSe2. In the presence of CDW order the quadrupolar interaction of the 93Nb nuclei with the local electric-fie
ld gradient is modified, and this in turn affects the magnetic dipolar coupling of the positive muon to these nuclei. For a weak magnetic field applied parallel to the c-axis, we observe a small enhancement of the muon depolarization rate at temperatures below the established CDW phase transition. Aligning the applied field perpendicular to the c-axis, we observe a sensivity to static CDW order in regions of the sample extending up to nearly 3 times the CDW transition temperature. The results suggest that the muon is mobile over the temperature range explored above the superconducting transition temperature (Tc), and becomes trapped in the vicinity of defects.
We have performed muon spin rotation/relaxation (muSR) measurements on single crystals of the chiral helimagnet Cr1/3NbS2 at zero to low magnetic field. The transition from the paramagnetic to helical magnetically ordered phase at zero field is marke
d by the onset of a coherent oscillation of the zero-field muon spin polarization below a critical temperature Tc. An enhancement of the muon spin precession frequency is observed below T ~ 50K, where anomalous behavior has been observed in bulk transport measurements. The enhanced precession frequency indicates a low-temperature modification of the helical magnetic structure. A Landau free energy analysis suggests that the low-temperature change in the magnetic structure is caused by a structural change, whereas the magnetic order above Tc is the result of an attractive interaction between the ferromagnetic moment induced by the applied field and the magnetic moments of the helical structure. We also suggest a longer periodicity of helicity below T ~ 50K, which can be verified by neutron scattering.
We report the results of a muon spin rotation (muSR) study of the bulk of Bi{2+x}Sr{2-x}CaCu2O{8+delta}, as well as pure and Ca-doped YBa2Cu3Oy, which together with prior measurements reveal a universal inhomogeneous magnetic-field response of hole-d
oped cuprates extending to temperatures far above the critical temperature (Tc). The primary features of our data are incompatible with the spatially inhomogeneous response being dominated by known charge density wave (CDW) and spin density wave (SDW) orders. Instead the normal-state inhomogeneous line broadening is found to scale with the maximum value Tc^max for each cuprate family, indicating it is controlled by the same energy scale as Tc. Since the degree of chemical disorder varies widely among the cuprates we have measured, the observed scaling constitutes evidence for an intrinsic electronic tendency toward inhomogeneity above Tc.
We report a high precision search for orbital-like magnetic order in the pseudogap region of La2-xSrxCuO4 single crystals using zero-field muon spin relaxation (ZF-muSR). In contrast to previous studies of this kind, the effects of the dipolar and qu
adrupolar interactions of the muon with nearby nuclei are calculated. ZF-muSR spectra with a high number of counts were also recorded to determine whether a magnetically ordered phase exists in dilute regions of the sample. Despite these efforts, we find no evidence for static magnetic order of any kind in the pseudogap region above the hole-doping concentration p = 0.13.
It is shown that attempts to accurately deduce the magnetic penetration depth of overdoped BaFe_{1.82}Co_{0.18}As2 single crystals by transverse-field muon spin rotation (TF-muSR) are thwarted by field-induced magnetic order and strong vortex-lattice
disorder. We explain how substantial deviations from the magnetic field distribution of a nearly perfect vortex lattice by one or both of these factors is also significant for other iron-based superconductors, and this introduces considerable uncertainty in the values of the magnetic penetration depth obtained by TF-muSR.
The doping of charge carriers into the CuO2 planes of copper oxide Mott insulators causes a gradual destruction of antiferromagnetism and the emergence of high-temperature superconductivity. Optimal superconductivity is achieved at a doping concentra
tion p beyond which further increases in doping cause a weakening and eventual disappearance of superconductivity. A potential explanation for this demise is that ferromagnetic fluctuations compete with superconductivity in the overdoped regime. In this case a ferromagnetic phase at very low temperatures is predicted to exist beyond the doping concentration at which superconductivity disappears. Here we report on a direct examination of this scenario in overdoped La2-xSrxCuO4 using the technique of muon spin relaxation. We detect the onset of static magnetic moments of electronic origin at low temperature in the heavily overdoped nonsuperconducting region. However, the magnetism does not exist in a commensurate long-range ordered state. Instead it appears as a dilute concentration of static magnetic moments. This finding places severe restrictions on the form of ferromagnetism that may exist in the overdoped regime. Although an extrinsic impurity cannot be absolutely ruled out as the source of the magnetism that does occur, the results presented here lend support to electronic band calculations that predict the occurrence of weak localized ferromagnetism at high doping.
We report that in YBa2Cu3Oy and La2-xSrxCuO4 there is a spatially inhomogeneous response to magnetic field for temperatures T extending well above the bulk superconducting transition temperature Tc. An inhomogeneous magnetic response is observed abov
e Tc even in ortho-II YBa2Cu3O6.50, which has highly ordered doping. The degree of the field inhomogeneity above Tc tracks the hole doping dependences of both Tc and the density of the superconducting carriers below Tc, and therefore is apparently coupled to superconductivity.
Highly disordered magnetism confined to individual weakly interacting vortices is detected by muon spin rotation in two different families of high-transition-temperature superconductors, but only in samples on the low-doping side of the low-temperatu
re normal state metal-to-insulator crossover (MIC). The results support an extended quantum phase transition (QPT) theory of competing magnetic and superconducting orders that incorporates the coupling between CuO2 planes. Contrary to what has been inferred from previous experiments, the static magnetism that coexists with superconductivity near the field-induced QPT is not ordered. Our findings unravel the mystery of the MIC and establish that the normal state of high-temperature superconductors is ubiquitously governed by a magnetic quantum critical point in the superconducting phase.
We report on muon spin rotation measurements of the internal magnetic field distribution n(B) in the vortex solid phase of YBa2Cu3Oy (YBCO) single crystals, from which we have simultaneously determined the hole doping dependences of the in-plane Ginz
burg-Landau (GL) length scales in the underdoped regime. We find that Tc has a sublinear dependence on 1/lambda_{ab}^2, where lambda_{ab} is the in-plane magnetic penetration depth in the extrapolated limits T -> 0 and H -> 0. The power coefficient of the sublinear dependence is close to that determined in severely underdoped YBCO thin films, indicating that the same relationship between Tc and the superfluid density is maintained throughout the underdoped regime. The in-plane GL coherence length (vortex core size) is found to increase with decreasing hole doping concentration, and exhibit a field dependence that is explained by proximity-induced superconductivity on the CuO chains. Both the magnetic penetration depth and the vortex core size are enhanced near 1/8 hole doping, supporting the belief by some that stripe correlations are a universal property of high-Tc cuprates.
