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A search for non-resonant D+(s) to pi+mu+mu- and D+(s) to pi-mu+mu+ decays is performed using proton-proton collision data, corresponding to an integrated luminosity of 1.0 fb-1, at sqrt(s) = 7 TeV recorded by the LHCb experiment in 2011. No signals are observed and the 90% (95%) confidence level (CL) limits on the branching fractions are B(D+ to pi+mu+mu-) < 7.3 (8.3) x 10-8, B(Ds+ to pi+mu+mu-) < 4.1 (4.8) x 10-7, B(D+ to pi-mu+mu+) < 2.2 (2.5) x 10-8, B(Ds+ to pi-mu+mu+) < 1.2 (1.4) x 10-7. These limits are the most stringent to date.
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