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In the course of investigations of thermal neutron detection based on mixtures of $^{10}$BF$_3$ with other gases, knowledge was required of the photoabsorption cross sections of $^{10}$BF$_3$ for wavelengths between 135 and 205 nm. Large discrepancie s in the values reported in existing literature led to the absolute measurements reported in this communication. The measurements were made at the SURF III synchrotron radiation facility at the National Institute of Standards and Technology. The measured absorption cross sections vary from 10$^{-20}$ cm$^2$ at 135 nm to less than 10$^{-21}$ cm$^2$ in the region from 165 to 205 nm. Three previously unreported absorption features with resolvable structure were found in the regions 135 to 145 nm, 150 to 165 nm and 190 to 205 nm. Quantum mechanical calculations, using the TD-B3LYP/aug-cc-pVDZ variant of time-dependent density functional theory implemented in Gaussian 09, suggest that the observed absorption features arise from symmetry-changing adiabatic transitions.
Previous work showed that the 3He(n,tp) reaction in a cell of 3He at atmospheric pressure generated tens of far-ultraviolet photons per reacted neutron. Here we report amplification of that signal by factors of 1000 and more when noble gases are adde d to the cell. Calibrated filter-detector measurements show that this large signal is due to noble-gas excimer emissions, and that the nuclear reaction energy is converted to far-ultraviolet radiation with efficiencies of up to 30%. The results have been placed on an absolute scale through calibrations at the NIST SURF III synchrotron. They suggest possibilities for high-efficiency neutron detectors as an alternative to existing proportional counters.
73 - L.Deng , E. W. Hagley , Qiang Cao 2010
We report the first experimental observations of strong suppression of matter-wave superradiance using blue-detuned pump light and demonstrate a pump-laser detuning asymmetry in the collective atomic recoil motion. In contrast to all previous theoret ical frameworks, which predict that the process should be symmetric with respect to the sign of the pump-laser detuning, we find that for condensates the symmetry is broken. With high condensate densities and red-detuned light, the familiar distinctive multi-order, matter-wave scattering pattern is clearly visible, whereas with blue-detuned light superradiance is strongly suppressed. In the limit of a dilute atomic gas, however, symmetry is restored.
We have detected Lyman alpha radiation as a product of the n(3He,t)p nuclear reaction occurring in a cell of 3He gas. The predominant source of this radiation appears to be decay of the 2p state of tritium produced by charge transfer and excitation c ollisions with the background 3He gas. Under the experimental conditions reported here we find yields of tens of Lyman alpha photons for every neutron reaction. These results suggest a method of cold neutron detection that is complementary to existing technologies that use proportional counters. In particular, this approach may provide single neutron sensitivity with wide dynamic range capability, and a class of neutron detectors that are compact and operate at relatively low voltages.
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