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130 - R. Wallauer , S. Sanna , E. Lahoud 2015
Angle-resolved photoemission spectroscopy (ARPES) is one of most powerful techniques to unravel the electronic properties of layered materials and in the last decades it has lead to a significant progress in the understanding of the band structures o f cuprates, pnictides and other materials of current interest. On the other hand, its application to Mott-Hubbard insulating materials where a Fermi surface is absent has been more limited. Here we show that in these latter materials, where electron spins are localized, ARPES may provide significant information on the spin correlations which can be complementary to the one derived from neutron scattering experiments. Sr$_2$Cu$_{1-x}$Zn$_x$O$_2$Cl$_2$, a prototype of diluted spin $S=1/2$ antiferromagnet (AF) on a square lattice, was chosen as a test case and a direct correspondence between the amplitude of the spectral weight beyond the AF zone boundary derived from ARPES and the spin correlation length $xi$ estimated from $^{35}$Cl NMR established. It was found even for correlation lengths of a few lattice constants a significant spectral weight in the back-bended band is present which depends markedly on $xi$. Moreover the temperature dependence of that spectral weight is found to scale with the $x$ dependent spin-stiffness. These findings prove that ARPES technique is very sensitive to short-range correlations and its relevance in the understanding of the electronic correlations in cuprates is discussed.
We measured the electronic structure of Fe substituted Bi2212 using Angle Resolved Photoemission Spectroscopy (ARPES). We find that the substitution does not change the momentum dependence of the superconducting gap but induces a very anisotropic enh ancement of the scattering rate. A comparison of the effect of Fe substitution to that of Zn substitution suggests that the Fe reduces T$_c$ so effectively because it supresses very strongly the coherence weight around the anti-nodes.
We report point contact measurements in high quality single crystals of Cu0.2Bi2Se3. We observe three different kinds of spectra: (1) Andreev-reflection spectra, from which we infer a superconducting gap size of 0.6mV; (2) spectra with a large gap wh ich closes above Tc at about 10K; and (3) tunneling-like spectra with zero-bias conductance peaks. These tunneling spectra show a very large gap of ~2meV (2Delta/KTc ~ 14).
We measured the electronic-structure of FeSe_xTe_1-x above and below Tc. In the normal state we find multiple bands with remarkably small values for the Fermi energy, E_F. Yet,below Tc we find a superconducting gap, Delta, that is comparable in size to E_F, leading to a ratio Delta/E_F~0.5 that is much larger than found in any previously studied superconductor. We also observe an anomalous dispersion of the coherence peak which is very similar to the dispersion found in cold Fermi-gas experiments and which is consistent with the predictions of the BCS-BEC crossover theory.
The phase diagram of the superconducting high-Tc cuprates is governed by two energy scales: T*, the temperature below which a gap is opened in the excitation spectrum, and Tc, the superconducting transition temperature. The way these two energy scale s are reflected in the low-temperature energy gap is being intensively debated. Using Zn substitution and carefully controlled annealing we prepared a set of samples having the same T* but different Tcs, and measured their gap using Angle Resolved Photoemission Spectroscopy (ARPES). We show that Tc is not related to the gap shape or size, but it controls the size of the coherence peak at the gap edge.
We report temperature- and magnetic field-dependent bulk muon spin rotation measurements in a c-axis oriented superconductor CaC6 in the mixed state. Using both a simple second moment analysis and the more precise analytical Ginzburg-Landau model, we obtained a field independent in-plane magnetic penetration depth {lambda}ab (0) = 72(3) nm. The temperature dependencies of the normalized muon spin relaxation rate and of the normalized superfluid density result to be identical, and both are well represented by the clean limit BCS model with 2Delta/kB Tc = 3.6(1), suggesting that CaC6 is a fully gapped BCS superconductor in the clean limit regime.
We report a comprehensive TF-muSR study of TiSe_2Cu_2. The magnetic penetration depth was found to saturate at low temperature as expected in an s-wave SC. As x is increased we find that the superfluid density increases and the size of the supercondu cting gap, calculated from the temperature dependence of the superfluid density, is approaching the BCS value. However, for low values of x, the gap is smaller than the weak-coupling BCS prediction suggesting that two superconducting gaps are present in the sample.
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