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The interplay among anisotropic magnetic terms, such as the bond-dependent Kitaev interactions and single-ion anisotropy, plays a key role in stabilizing the finite-temperature ferromagnetism in the two-dimensional compound $rm{CrSiTe_3}$. While the Heisenberg interaction is predominant in this material, a recent work shows that it is rather sensitive to the compressive strain, leading to a variety of phases, possibly including a sought-after Kitaev quantum spin liquid [C. Xu, textit{et. al.}, Phys. Rev. Lett. textbf{124}, 087205 (2020)]. To further understand these states, we establish the quantum phase diagram of a related bond-directional spin-$3/2$ model by the density-matrix renormalization group method. As the Heisenberg coupling varies from ferromagnetic to antiferromagnetic, three magnetically ordered phases, i.e., a ferromagnetic phase, a $120^circ$ phase and an antiferromagnetic phase, appear consecutively. All the phases are separated by first-order phase transitions, as revealed by the kinks in the ground-state energy and the jumps in the magnetic order parameters. However, no positive evidence of the quantum spin liquid state is found and possible reasons are discussed briefly.
The dependence of high-harmonic generation (HHG) on laser ellipticity is investigated using a modified ZnO model. In the driving of relatively weak field, we reproduce qualitatively the ellipticity dependence as observed in the HHG experiment of wurt zite ZnO. When increasing the field strength, the HHG shows an anomalous ellipticity dependence, similar to that observed experimentally in the single-crystal MgO. With the help of a semiclassical analysis, it is found that the key mechanism inducing the change of ellipticity dependence is the interplay between the dynamical Bloch oscillation and the anisotropic band structure. The dynamical Bloch oscillation contributes additional quantum paths, which are less sensitive to ellipticity. The anisotropic band-structure make the driving pulse with finite ellipticity be able to drive the pairs to the band positions with larger gap, which extends the harmonic cutoff. The combination of these two effects leads to the anomalous ellipticity dependence. The result reveals the importance of dynamical Bloch oscillations for the ellipticity dependence of HHG from bulk ZnO.
Motivated by the recent experiment on $rm{K_2Cu_3Oleft(SO_4right)_3}$, an edge-shared tetrahedral spin-cluster compound [M. Fujihala textit{et al.}, Phys. Rev. Lett. textbf{120}, 077201 (2018)], we investigate two-leg spin-cluster ladders with the pl aquette number $n_p$ in each cluster up to six by the density-matrix renormalization group method. We find that the phase diagram of such ladders strongly depends on the parity of $n_p$. For even $n_p$, the phase diagram has two phases, one is the Haldane phase, and the other is the cluster rung-singlet phase. For odd $n_p$, there are four phases, which are a cluster-singlet phase, a cluster rung-singlet phase, a Haldane phase and an even Haldane phase. Moreover, in the latter case the region of the Haldane phase increases while the cluster-singlet phase and the even Haldane phase shrink as $n_p$ increases. We thus conjecture that in the large $n_p$ limit, the phase diagram will become independent of $n_p$. By analysing the ground-state energy and entanglement entropy we obtain the order of the phase transtions. In particular, for $n_p=1$ there is no phase transition between the even Haldane phase and the cluster-singlet phase while for other odd $n_p$ there is a first-order phase transition. Our work provides comprehensive phase diagrams for these cluster-based models and may be helpful to understand experiments on related materials.
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