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We performed temperature dependent X-ray linear dichroism (XLD) experiments on an iron pnictide system, Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ with $x$=0.00 and 0.05, to experimentally verify existence of orbital ordering (OO). We observed clear XLD in polar ization dependent X-ray absorption spectra of Fe $L$ edges. By exploiting the difference in the temperature dependent behaviors, we were able to separate OO and structure contributions to XLD. The observed OO signal indicates different occupation numbers for $d_{yz}$ and $d_{zx}$ orbitals and supports existence of a ferro-OO. The results are also consistent with the theoretical prediction. Moreover, we find substantial OO signal above the transition temperature, which suggests that OO fluctuation exists well above the transition temperature.
152 - Y. K. Kim , Hyungju Oh , Chul Kim 2010
We performed angle resolved photoelectron spectroscopy (ARPES) studies on mechanically detwinned BaFe2As2. We observe clear band dispersions and the shapes and characters of the Fermi surfaces are identified. Shapes of the two hole pockets around the {Gamma}-point are found to be consistent with the Fermi surface topology predicted in the orbital ordered states. Dirac-cone like band dispersions near the {Gamma}-point are clearly identified as theoretically predicted. At the X-point, split bands remain intact in spite of detwinning, barring twinning origin of the bands. The observed band dispersions are compared with calculated band structures. With a magnetic moment of 0.2 ?B per iron atom, there is a good agreement between the calculation and experiment.
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