Pb films embedded with homogeneously distributed cobalt (Co) nanoparticles (mean size 4.5 nm) have been prepared. Previous transport investigations have shown that Co particles induce spontaneous vortices below the superconducting transition temperat
ure (T$_{c}$) in zero external magnetic field. In this paper we study in detail the influence of the Co volume franction and an external magnetic field on the superconducting transition in such composites. The large difference in T$_c$-reduction between the as-prepared and annealed samples can be attributed to the different superconducting coherence lengths and the resulting different diameters of the spontaneous vortices in these samples.
A hybrid system which consists of a superconducting (SC) Pb film (100 nm thickness) containing $sim$1 vol% single domain ferromagnetic (FM) Co particles of mean-size $sim$4.5 nm reveal unusual magnetic properties: (i) a controlled switching between t
he usual diamagnetic and the unusual paramagnetic Meissner effect in field cooling as well as in zero-field cooling experiments (ii) amplification of the positive magnetization when the sample enters the SC state below T$_c$. These experimental findings can be explained by the formation of spontaneous vortices and the possible alignment of these vortices due to the foregoing alignment of the Co particle FM moments by an external magnetic field.
The interplay between superconductivity and magnetism gives rise to many intriguing and exciting phenomena. In this Letter we report about a novel manifestation of this interplay: a temperature induced phase transition between different spontaneous v
ortex phases in lead superconducting films with embedded magnetic nanoparticles. Unlike common vortices in superconductors the vortex phase appears without any applied magnetic field. The vortices nucleate exclusively due to the stray field of the magnetic nanoparticles, which serve the dual role of providing the internal field and simultaneously acting as pinning centers. As in usual superconductors, one can move the spontaneous vortices with an applied electric current. Transport measurements reveal dynamical phase transitions that depend on temperature (T) and applied field (H) and support the obtained (H-T) phase diagram. In particular, we used a scaling analysis to characterize a transition from a liquid to a novel disordered solid resembling a vortex glass.
