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In recent years, it has been shown that Berry curvature monopoles and dipoles play essential roles in the anomalous Hall effect and the nonlinear Hall effect respectively. In this work, we demonstrate that Berry curvature multipoles (the higher momen ts of Berry curvatures at the Fermi energy) can induce higher-order nonlinear anomalous Hall (NLAH) effect. Specifically, an AC Hall voltage perpendicular to the current direction emerges, where the frequency is an integer multiple of the frequency of the applied current. Importantly, by analyzing the symmetry properties of all the 3D and 2D magnetic point groups, we note that the quadrupole, hexapole and even higher Berry curvature moments can cause the leading-order frequency multiplication in certain materials. To provide concrete examples, we point out that the third-order NLAH voltage can be the leading-order Hall response in certain antiferromagnets due to Berry curvature quadrupoles, and the fourth-order NLAH voltage can be the leading response in the surface states of topological insulators induced by Berry curvature hexapoles. Our results are established by symmetry analysis, effective Hamiltonian and first-principles calculations. Other materials which support the higher-order NLAH effect are further proposed, including 2D antiferromagnets and ferromagnets, Weyl semimetals and twisted bilayer graphene near the quantum anomalous Hall phase.
In this work, we demonstrate that making a cut (a narrow vacuum regime) in the bulk of a quantum anomalous Hall insulator (QAHI) creates a topologically protected single helical channel with counter-propagating electron modes, and inducing supercondu ctivity on the helical channel through proximity effect will create Majorana zero energy modes (MZMs) at the ends of the cut. In this geometry, there is no need for the proximity gap to overcome the bulk insulating gap of the QAHI to create MZMs as in the two-dimensional QAHI/superconductor (QAHI/SC) heterostructures. Therefore, the topological regime with MZMs is greatly enlarged. Furthermore, due to the presence of a single helical channel, the generation of low energy in-gap bound states caused by multiple conducting channels is avoided such that the MZMs can be well separated from other in-gap excitations in energy. This simple but practical approach allows the creation of a large number of MZMs in devices with complicated geometry such as hexons for measurement-based topological quantum computation. We further demonstrate how braiding of MZMs can be performed by controlling the coupling strength between the counter-propagating electron modes.
Recently, it was pointed out that all chiral crystals with spin-orbit coupling (SOC) can be Kramers Weyl semimetals (KWSs) which possess Weyl points pinned at time-reversal invariant momenta. In this work, we show that all achiral non-centrosymmetric materials with SOC can be a new class of topological materials, which we term Kramers nodal line metals (KNLMs). In KNLMs, there are doubly degenerate lines, which we call Kramers nodal lines (KNLs), connecting time-reversal invariant momenta. The KNLs create two types of Fermi surfaces, namely, the spindle torus type and the octdong type. Interestingly, all the electrons on octdong Fermi surfaces are described by two-dimensional massless Dirac Hamiltonians. These materials support quantized optical conductance in thin films. We further show that KNLMs can be regarded as parent states of KWSs. Therefore, we conclude that all non-centrosymmetric metals with SOC are topological, as they can be either KWSs or KNLMs.
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