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We use neutron resonance spin echo and Larmor diffraction to study the effect of uniaxial pressure on the tetragonal-to-orthorhombic structural ($T_s$) and antiferromagnetic (AF) phase transitions in iron pnictides BaFe$_{2-x}$Ni$_{x}$As$_{2}$ ($x=0, 0.03,0.12$), SrFe$_{1.97}$Ni$_{0.03}$As$_2$, and BaFe$_2$(As$_{0.7}$P$_{0.3}$)$_2$. In antiferromagnetically ordered BaFe$_{2-x}$Ni$_{x}$As$_{2}$ and SrFe$_{1.97}$Ni$_{0.03}$As$_2$ with $T_N$ and $T_s$ ($T_Nleq T_s$), a uniaxial pressure necessary to detwin the sample also increases $T_N$, smears out the structural transition, and induces an orthorhombic lattice distortion at all temperatures. By comparing temperature and doping dependence of the pressure induced lattice parameter changes with the elastoresistance and nematic susceptibility obtained from transport and ultrasonic measurements, we conclude that the in-plane resistivity anisotropy found in the paramagnetic state of electron underdoped iron pnictides depends sensitively on the nature of the magnetic phase transition and a strong coupling between the uniaxial pressure induced lattice distortion and electronic nematic susceptibility.
We use inelastic neutron scattering (INS) to study the spin excitations in partially detwinned NaFe$_{0.985}$Co$_{0.015}$As which has coexisting static antiferromagnetic (AF) order and superconductivity ($T_c=15$ K, $T_N=30$ K). In previous INS work on a twinned sample, spin excitations form a dispersive sharp resonance near $E_{r1}=3.25$ meV and a broad dispersionless mode at $E_{r1}=6$ meV at the AF ordering wave vector ${bf Q}_{rm AF}={bf Q}_1=(1,0)$ and its twinned domain ${bf Q}_2=(0,1)$. For partially detwinned NaFe$_{0.985}$Co$_{0.015}$As with the static AF order mostly occurring at ${bf Q}_{rm AF}=(1,0)$, we still find a double resonance at both wave vectors with similar intensity. Since ${bf Q}_1=(1,0)$ characterizes the explicit breaking of the spin rotational symmetry associated with the AF order, these results indicate that the double resonance cannot be due to the static and fluctuating AF orders, but originate from the superconducting gap anisotropy.
We report elastic neutron scattering and transport measurements on the Ni and Cr equivalently doped iron pnictide BaFe$_{2-2x}$Ni$_{x}$Cr$_{x}$As$_{2}$. Compared with the electron-doped BaFe$_{2-x}$Ni$_{x}$As$_{2}$, the long-range antiferromagnetic ( AF) order in BaFe$_{2-2x}$Ni$_{x}$Cr$_{x}$As$_{2}$ is gradually suppressed with vanishing ordered moment and N{e}el temperature near $x= 0.20$ without the appearance of superconductivity. A detailed analysis on the transport properties of BaFe$_{2-x}$Ni$_{x}$As and BaFe$_{2-2x}$Ni$_{x}$Cr$_{x}$As$_{2}$ suggests that the non-Fermi-liquid behavior associated with the linear resistivity as a function of temperature may not correspond to the disappearance of the static AF order. From the temperature dependence of the resistivity in overdoped compounds without static AF order, we find that the transport properties are actually affected by Cr impurity scattering, which may induce a metal-to-insulator crossover in highly doped BaFe$_{1.7-y}$Ni$_{0.3}$Cr$_{y}$As$_{2}$.
Understanding the microscopic origins of electronic phases in high-transition temperature (high-Tc) superconductors is important for elucidating the mechanism of superconductivity. In the paramagnetic tetragonal phase of BaFe2-xTxAs2 (where T is Co o r Ni) iron pnictides, an in-plane resistivity anisotropy has been observed. Here we use inelastic neutron scattering to show that low-energy spin excitations in these materials change from four-fold symmetric to two-fold symmetric at temperatures corresponding to the onset of the in-plane resistivity anisotropy. Because resistivity and spin excitation anisotropies both vanish near optimal superconductivity, we conclude that they are likely intimately connected.
We use inelastic neutron scattering to study the effect of an in-plane magnetic field on the magnetic resonance in optimally doped superconductors FeSe$_{0.4}$Te$_{0.6}$ ($T_c=14$ K) and BaFe$_{1.9}$Ni$_{0.1}$As$_{2}$ ($T_c=20$ K). While the magnetic field up to 14.5 Tesla does not change the energy of the resonance, it particially suppresses $T_c$ and the corresponding superconductivity-induced intensity gain of the mode. However, we find no direct evidence for the field-induced spin-1 Zeeman splitting of the resonance. Therefore, it is still unclear if the resonance is the long-sought singlet-triplet excitation directly coupled to the superconducting electron Cooper pairs.
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