Experimental studies of high-purity kagome-lattice antiferromagnets (KAFM) are of great importance in attempting to better understand the predicted enigmatic quantum spin-liquid ground state of the KAFM model. However, realizations of this model can
rarely evade magnetic ordering at low temperatures due to various perturbations to its dominant isotropic exchange interactions. Such a situation is for example encountered due to sizable Dzyaloshinskii-Moriya magnetic anisotropy in YCu$_3$(OH)$_6$Cl$_3$, which stands out from other KAFM materials by its perfect crystal structure. We find evidence of magnetic ordering also in the distorted sibling compound Y$_3$Cu$_9$(OH)$_{18}$[Cl$_8$(OH)], which has recently been proposed to feature a spin-liquid ground state arising from a spatially anisotropic kagome lattice. Our findings are based on a combination of bulk susceptibility, specific heat, and magnetic torque measurements that disclose a Neel transition temperature of $T_N=11$~K in this material, which might feature a coexistence of magnetic order and persistent spin dynamics as previously found in YCu$_3$(OH)$_6$Cl$_3$. Contrary to previous studies of single crystals and powders containing impurity inclusions, we use high-purity single crystals of Y$_3$Cu$_9$(OH)$_{18}$[Cl$_8$(OH)] grown via an optimized hydrothermal synthesis route that minimizes such inclusions. This study thus demonstrates that the lack of magnetic ordering in less pure samples of the investigated compound does not originate from the reduced symmetry of spin lattice but is instead of extrinsic origin.
[Background] Predictions of spectroscopic properties of low-lying states are critical for nuclear structure studies. Theoretical methods can be particularly involved for odd-mass nuclei because of the interplay between the unpaired nucleon and collec
tive degrees of freedom. Only a few models have been developed for systems in which octupole collective degrees of freedom play a role. [Purpose] We aim to predict spectroscopic properties of odd-mass nuclei characterized by octupole shape deformation, employing a model that describes single-particle and collective degrees of freedom within the same microscopic framework. [Method] A microscopic core-quasiparticle coupling (CQC) model based on the covariant density functional theory is developed, which includes collective excitations of even-mass core nuclei and single-particle states of the odd nucleon, calculated using a quadrupole-octupole collective Hamiltonian combined with a constrained reflection-asymmetric relativistic Hartree-Bogoliubov model. [Results] Model predictions for low-energy excitation spectra and transition rates of odd-mass radium isotopes $^{223, 225, 227}$Ra are shown to be in good agreement with available data. [Conclusions] A microscopic CQC model based on covariant density functional theory has been developed for odd-mass nuclei characterized by both quadrupole and octupole shape deformations. Theoretical results reproduce data in odd-mass Ra isotopes and provide useful predictions for future studies of octupole correlations in nuclei and related phenomena.
This paper analyzes turbulence-chemistry interactions for an n-dodecane-air flame, focusing on the degree to which fuel oxidation pathways change in turbulent flames relative to their corresponding laminar flames. This work is based on a lean n-dodec
ane-air flame DNS database from Aspden et al. (Proc. Combust. Institute, 36 (2017) 2005-2016). The relative roles of dominant reactions that release heat and produce/consume radicals are examined at various turbulence intensities and compared with stretched flame calculations from counterflow flames and perfectly stirred reactors. These results show that spatially integrated (i.e. integrated heat release or radical production rate metrics averaged over the entire flame) chemical pathways are relatively insensitive to turbulence intensity and mimic the behavior of stretched flames. In other words, the contribution of a given reaction to heat release or radical production, integrated over the entire flame, is nearly independent to turbulence. Localized analysis conditioned on topological feature of the flame and on temperature is also performed. The former analysis reveals that much larger alteration of pathways occurs in the positively-curved regions of the flame. The latter localized analysis shows that peak activity in the low temperature (i.e. below 1200K) region shift towards higher temperatures with increases in Karlovitz number. This result is particularly interesting given that prior work with lighter fuels showed the opposite behavior suggesting a disparate response of the reactions involved in the fuel oxidation process to increased turbulence.
Recent experiments showed that Co undergoes a phase transition from ferromagnetic hcp phase to non-magnetic fcc one around 100 GPa. Since the transition is of first order, a certain region of co-existence of the two phases is present. By means of tex
tit{ab initio} calculations, we found that the hcp phase itself undergoes a series of electronic topological transitions (ETTs), which affects both elastic and magnetic properties of the material. Most importantly, we propose that the sequence of ETTs lead to the stabilisation of a non-collinear spin arrangement in highly compressed hcp Co. Details of this non-collinear magnetic state and the interatomic exchange parameters that are connected to it, are presented here.
Plasmon mode in a silver nanowire is theoretically studied when the nanowire is placed on or near a silica substrate. It is found that the substrate has much influence on the plasmon mode. For the nanowire on the substrate, the plasmon (hybrid) mode
possesses not only a long propagation length but also an ultrasmall mode area. From the experimental point of view, this cavity-free structure holds a great potential to study a strong coherent interaction between the plasmon mode and single quantum system (for example, quantum dots) embedded in the substrate.
The indistinguishability of independent single photons is presented by decomposing the single photon pulse into the mixed state of different transform limited pulses. The entanglement between single photons and outer environment or other photons indu
ces the distribution of the center frequencies of those transform limited pulses and makes photons distinguishable. Only the single photons with the same transform limited form are indistinguishable. In details, the indistinguishability of single photons from the solid-state quantum emitter and spontaneous parametric down conversion is examined with two-photon Hong-Ou-Mandel interferometer. Moreover, experimental methods to enhance the indistinguishability are discussed, where the usage of spectral filter is highlighted.
We describe and examine entanglement between different degrees of freedom in multiphoton states based on the permutation properties. From the state description, the entanglement comes from the permutation asymmetry. According to the different permuta
tion properties, the multiphoton states can be divided into several parts. It will help to deal with the multiphoton interference, which can be used as the measurement of the entanglement.
In this paper, photonic entanglement and interference are described and analyzed with the language of quantum information process. Correspondingly, a photon state involving several degrees of freedom is represented in a new expression based on the pe
rmutation symmetry of bosons. In this expression, each degree of freedom of a single photon is regarded as a qubit and operations on photons as qubit gates. The two-photon Hong-Ou-Mandel interference is well interpreted with it. Moreover, the analysis reveals the entanglement between different degrees of freedom in a four-photon state from parametric down conversion, even if there is no entanglement between them in the two-photon state. The entanglement will decrease the state purity and photon interference visibility in the experiments on a four-photon polarization state.
We construct a linear optics measurement process to determine the entanglement measure, named emph{I-concurrence}, of a set of $4 times 4$ dimensional two-photon entangled pure states produced in the optical parametric down conversion process. In our
experiment, an emph{equivalent} symmetric projection for the two-fold copy of single subsystem (presented by L. Aolita and F. Mintert, Phys. Rev. Lett. textbf{97}, 050501 (2006)) can be realized by observing the one-side two-photon coincidence without any triggering detection on the other subsystem. Here, for the first time, we realize the measurement for entanglement contained in bi-photon pure states by taking advantage of the indistinguishability and the bunching effect of photons. Our method can determine the emph{I-concurrence} of generic high dimensional bipartite pure states produced in parametric down conversion process.
We propose and demonstrate experimentally a projection scheme to measure the quantum phase with a precision beating the standard quantum limit. The initial input state is a twin Fock state $|N,N>$ proposed by Holland and Burnett [Phys. Rev. Lett. {bf
71}, 1355 (1993)] but the phase information is extracted by a quantum state projection measurement. The phase precision is about $1.4/N$ for large photon number $N$, which approaches the Heisenberg limit of 1/N. Experimentally, we employ a four-photon state from type-II parametric down-conversion and achieve a phase uncertainty of $0.291pm 0.001$ beating the standard quantum limit of $1/sqrt{N} = 1/2$ for four photons.
