We predict the non-linear non-equilibrium response of a magnetolyte, the Coulomb fluid of magnetic monopoles in spin ice. This involves an increase of the monopole density due to the second Wien effect---a universal and robust enhancement for Coulomb
systems in an external field---which in turn speeds up the magnetization dynamics, manifest in a non-linear susceptibility. Along the way, we gain new insights into the AC version of the classic Wien effect. One striking discovery is that of a frequency window where the Wien effect for magnetolyte and electrolyte are indistinguishable, with the former exhibiting perfect symmetry between the charges. In addition, we find a new low-frequency regime where the growing magnetization counteracts the Wien effect. We discuss for what parameters best to observe the AC Wien effect in Dy$_2$Ti$_2$O$_7$.
The Second Wien Effect describes the non-linear, non-equilibrium response of a weak electrolyte in moderate to high electric fields. Onsagers 1934 electrodiffusion theory along with various extensions has been invoked for systems and phenomena as div
erse as solar cells, surfactant solutions, water splitting reactions, dielectric liquids, electrohydrodynamic flow, water and ice physics, electrical double layers, non-Ohmic conduction in semiconductors and oxide glasses, biochemical nerve response and magnetic monopoles in spin ice. In view of this technological importance and the experimental ubiquity of such phenomena, it is surprising that Onsagers Wien effect has never been studied by numerical simulation. Here we present simulations of a lattice Coulomb gas, treating the widely applicable case of a double equilibrium for free charge generation. We obtain detailed characterisation of the Wien effect and confirm the accuracy of the analytical theories as regards the field evolution of the free charge density and correlations. We also demonstrate that simulations can uncover further corrections, such as how the field-dependent conductivity may be influenced by details of microscopic dynamics. We conclude that lattice simulation offers a powerful means by which to investigate system-specific corrections to the Onsager theory, and thus constitutes a valuable tool for detailed theoretical studies of the numerous practical applications of the Second Wien Effect.
