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We investigate the many-body effects of a magnetic adatom in ferromagnetic graphene by using the numerical renormalization group method. The nontrivial band dispersion of ferromagnetic graphene gives rise to interesting Kondo physics different from t hat in conventional ferromagnetic materials. For a half-filled impurity in undoped graphene, the presence of ferromagnetism can bring forth Kondo correlations, yielding two kink structures in the local spectral function near the Fermi energy. When the spin splitting of local occupations is compensated by an external magnetic field, the two Kondo kinks merge into a full Kondo resonance characterizing the fully screened ground state. Strikingly, we find the resulting Kondo temperature monotonically increases with the spin polarization of Dirac electrons, which violates the common sense that ferromagnetic bands are usually detrimental to Kondo correlations. Doped ferromagnetic graphene can behave as half metals, where its density of states at the Fermi energy linearly vanishes for one spin direction but keeps finite for the opposite direction. In this regime, we demonstrate an abnormal Kondo resonance that occurs in the first spin direction, while completely absent in the other one.
73 - Tie-Feng Fang , Ai-Min Guo , 2018
We investigate Kondo correlations in a quantum dot with normal and superconducting electrodes, where a spin bias voltage is applied across the device and the local interaction $U$ is either attractive or repulsive. When the spin current is blockaded in the large-gap regime, this nonequilibrium strongly-correlated problem maps into an equilibrium model solvable by the numerical renormalization group method. The Kondo spectra with characteristic splitting due to the nonequilibrium spin accumulation are thus obtained at high precision. It is shown that while the bias-induced decoherence of the spin Kondo effect is partially compensated by the superconductivity, the charge Kondo effect is enhanced out of equilibrium and undergoes an additional splitting by the superconducting proximity effect, yielding four Kondo peaks in the local spectral density. In the charge Kondo regime, we find a universal scaling of charge conductance in this hybrid device under different spin biases. The universal conductance as a function of the coupling to the superconducting lead is peaked at and hence directly measures the Kondo temperature. Our results are of direct relevance to recent experiments realizing negative-$U$ charge Kondo effect in hybrid oxide quantum dots [Nat. Commun. textbf{8}, 395 (2017)].
A quantum dot formed in a suspended carbon nanotube exposed to an external magnetic field is predicted to act as a thermoelectric unipolar spin battery which generates pure spin current. The built-in spin flip mechanism is a consequence of the spin-v ibration interaction resulting from the interplay between the intrinsic spin-orbit coupling and the vibrational modes of the suspended carbon nanotube. On the other hand, utilizing thermoelectric effect, the temperature difference between the electron and the thermal bath to which the vibrational modes are coupled provides the driving force. We find that both magnitude and direction of the generated pure spin current are dependent on the strength of spin-vibration interaction, the sublevel configuration in dot, the temperatures of electron and thermal bath, and the tunneling rate between the dot and the pole. Moreover, in the linear response regime, the kinetic coefficient is non-monotonic in the temperature $T$ and it reaches its maximum when $k_BT$ is about one phonon energy. The existence of a strong intradot Coulomb interaction is irrelevant for our spin battery, provided that high-order cotunneling processes are suppressed.
Phonon-assisted electronic tunnelings through a vibrating quantum dot embedded between normal and superconducting leads are studied in the Kondo regime. In such a hybrid device, with the bias applied to the normal lead, we find a series of Kondo side bands separated by half a phonon energy in the differential conductance, which are distinct from the phonon-assisted sidebands previously observed in the conventional Andreev tunnelings and in systems with only normal leads. These Kondo sidebands originate from the Kondo-Andreev cooperative cotunneling mediated by phonons, which exhibit a novel Kondo transport behavior due to the interplay of the Kondo effect, the Andreev tunnelings, and the mechanical vibrations. Our result could be observed in a recent experiment setup [J. Gramich emph{et al.}, PRL textbf{115}, 216801 (2015)], provided that their carbon nanotube device reaches the Kondo regime at low temperatures.
40 - Lin Li , Zhan Cao , Tie-Feng Fang 2015
Motivated by experimental observation of the Kondo-enhanced Andreev transport [R. S. Deacon textit{et al.}, PRB textbf{81}, 121308(R) (2010)] in a hybrid normal metal-quantum dot-superconductor (N-QD-S) device, we theoretically study the Kondo effect in such a device and clarify the different roles played by the normal and superconducting leads. Due to the Andreev reflection in a QD-S system, a pair of Andreev energy levels form in the superconducting gap, which is able to carry the magnetic moment if the ground state of the QD is a magnetic doublet. In this sense, the Andreev energy levels play a role of effective impurity levels. When the normal lead is coupled to the QD-S system, on the one hand, the Andreev energy levels broaden to form the so-called Andreev bound states (ABSs), on the other hand, it can screen the magnetic moment of the ABSs. By tuning the couplings between the QD and the normal (superconducting) leads, the ABSs can simulate the Kondo, mixed-valence, and even empty orbit regimes of the usual single-impurity Anderson model. The above picture is confirmed by the Greens function calculation of the hybrid N-QD-S Anderson model and is also able to explain qualitatively experimental phenomena observed by Deacon textit{et al.}. These results can further stimulate related experimental study in the N-QD-S systems.
91 - Zhan Cao , Tie-Feng Fang , Lin Li 2015
Thermoelectric effect is exploited to optimize the Cooper pair splitting efficiency in a Y-shaped junction, which consists of two normal leads coupled to an $s$-wave superconductor via double noninteracting quantum dots. Here, utilizing temperature d ifference rather than bias voltage between the two normal leads, and tuning the two dot levels such that the transmittance of elastic cotunneling process is particle-hole symmetric, we find currents flowing through the normal leads are totally contributed from the splitting of Cooper pairs emitted from the superconductor. Such a unitary splitting efficiency is significantly better than the efficiencies obtained in experiments so far.
Spin susceptibility of Anderson impurities is a key quantity in understanding the physics of Kondo screening. Traditional numerical renormalization group (NRG) calculation of the impurity contribution $chi_{textrm{imp}}$ to susceptibility, defined or iginally by Wilson in a flat wide band, has been generalized before to structured conduction bands. The results brought about non-Fermi-liquid and diamagnetic Kondo behaviors in $chi_{textrm{imp}}$, even when the bands are not gapped at the Fermi energy. Here, we use the full density-matrix (FDM) NRG to present high-quality data for the local susceptibility $chi_{textrm{loc}}$ and to compare them with $chi_{textrm{imp}}$ obtained by the traditional NRG. Our results indicate that those exotic behaviors observed in $chi_{textrm{imp}}$ are unphysical. Instead, the low-energy excitations of the impurity in arbitrary bands only without gap at the Fermi energy are still a Fermi liquid and paramagnetic. We also demonstrate that unlike the traditional NRG yielding $chi_{textrm{loc}}$ less accurate than $chi_{textrm{imp}}$, the FDM method allows a high-precision dynamical calculation of $chi_{textrm{loc}}$ at much reduced computational cost, with an accuracy at least one order higher than $chi_{textrm{imp}}$. Moreover, artifacts in the FDM algorithm to $chi_{textrm{imp}}$, and origins of the spurious non-Fermi-liquid and diamagnetic features are clarified. Our work provides an efficient high-precision algorithm to calculate the spin susceptibility of impurity for arbitrary structured bands, while negating the applicability of Wilsons definition to such cases.
97 - Zhan Cao , Tie-Feng Fang , 2014
We propose a scheme to detect the Majorana bound states (MBSs) by a thermodynamically stable D.C. Josephson current with $4pi$-periodicity in the superconducting phase difference, which is distinct from the previous A.C. $4pi$-periodicity found in to pological superconducting Josephson junctions. The scheme, consisting of a quantum dot coupled to two s-wave superconducting leads and a floating topological superconductor supporting two MBSs at its ends, only exploits the interplay of a local Zeeman field and the exotic helical and self-Hermitian properties of MBSs, without requiring the conservation of fermion parity and not relying on the zero-energy property of MBSs. Our D.C. $4pi$-periodicity is thus robust against the overlap between the two MBSs and various system parameters, including the local Coulomb interaction, the tunneling asymmetry, and the width of superconducting gap, which facilitates experimentally detection of the MBSs.
We investigate single-electron transport through quantum dots with negative charging energy induced by a polaronic energy shift. For weak dot-lead tunnel couplings, we demonstrate a bipolaronic blockade effect at low biases which suppresses the oscil lating linear conductance, while the conductance resonances under large biases are enhanced. Novel conductance plateau develops when the coupling asymmetry is introduced, with its height and width tuned by the coupling strength and external magnetic field. It is further shown that the amplitude ratio of magnetic-split conductance peaks changes from 3 to 1for increasing coupling asymmetry. Though we demonstrate all these transport phenomena in the low-order single-electron tunneling regime, they are already strikingly different from the usual Coulomb blockade physics and are easy to observe experimentally.
We propose carbon nanotubes (CNTs) with magnetic impurities as a versatile platform to achieve unconventional Kondo physics, where the CNT bath is gapped by the spin-orbit interaction and surface curvature. While the strong-coupling phase is inaccess ible for the special case of half-filled impurities in neutral armchair CNTs, the system in general can undergo quantum phase transitions to the Kondo ground state. The resultant position-specific phase diagrams are investigated upon variation of the CNT radius, chirality, and carrier doping, revealing several striking features, e.g., the existence of a maximal radius for nonarmchair CNTs to realize phase transitions, and an interference-induced suppression of the Kondo screening. We show that by tuning the Fermi energy via electrostatic gating, the quantum critical region can be experimentally accessed.
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