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When an atom strongly couples to a cavity, it can undergo coherent vacuum Rabi oscillations. Controlling these oscillatory dynamics quickly relative to the vacuum Rabi frequency enables remarkable capabilities such as Fock state generation and determ inistic synthesis of quantum states of light, as demonstrated using microwave frequency devices. At optical frequencies, however, dynamical control of single-atom vacuum Rabi oscillations remains challenging. Here, we demonstrate coherent transfer of optical frequency excitation between a single quantum dot and a cavity by controlling vacuum Rabi oscillations. We utilize a photonic molecule to simultaneously attain strong coupling and a cavity-enhanced AC Stark shift. The Stark shift modulates the detuning between the two systems on picosecond timescales, faster than the vacuum Rabi frequency. We demonstrate the ability to add and remove excitation from the cavity, and perform coherent control of light-matter states. These results enable ultra-fast control of atom-cavity interactions in a nanophotonic device platform.
We present a method to control the resonant coupling interaction in a coupled-cavity photonic crystal molecule by using a local and reversible photochromic tuning technique. We demonstrate the ability to tune both a two-cavity and a three-cavity phot onic crystal molecule through the resonance condition by selectively tuning the individual cavities. Using this technique, we can quantitatively determine important parameters of the coupled-cavity system such as the photon tunneling rate. This method can be scaled to photonic crystal molecules with larger numbers of cavities, which provides a versatile method for studying strong interactions in coupled resonator arrays.
We demonstrate a method of tuning a semiconductor quantum dot (QD) onto resonance with a cavity mode all-optically. We use a system comprised of two evanescently coupled cavities containing a single QD. One resonance of the coupled cavity system is u sed to generate a cavity enhanced optical Stark shift, enabling the QD to be resonantly tuned to the other cavity mode. A twenty-seven fold increase in photon emission from the QD is measured when the off-resonant QD is Stark shifted into the cavity mode resonance, which is attributed to radiative enhancement of the QD. A maximum tuning of 0.06 nm is achieved for the QD at an incident power of 88 {mu}W.
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