Measurements of sulphur isotopes in presolar grains can help to identify the astrophysical sites in which these grains were formed. A more precise thermonuclear rate of the 33S(p,gamma)34Cl reaction is required, however, to assess the diagnostic abil
ity of sulphur isotopic ratios. We have studied the 33S(3He,d)34Cl proton-transfer reaction at 25 MeV using a high-resolution quadrupole-dipole-dipole-dipole magnetic spectrograph. Deuteron spectra were measured at ten scattering angles between 10 and 55 degrees. Twenty-four levels in 34Cl over Ex = 4.6 - 5.9 MeV were observed, including three levels for the first time. Proton spectroscopic factors were extracted for the first time for levels above the 33S+p threshold, spanning the energy range required for calculations of the thermonuclear 33S(p,gamma)34Cl rate in classical nova explosions. We have determined a new 33S(p,gamma)34Cl rate using a Monte Carlo method and have performed new hydrodynamic nova simulations to determine the impact on nova nucleosynthesis of remaining nuclear physics uncertainties in the reaction rate. We find that these uncertainties lead to a factor of less than 5 variation in the 33S(p,gamma)34Cl rate over typical nova peak temperatures, and variation in the ejected nova yields of S--Ca isotopes by less than 20%. In particular, the predicted 32S/33S ratio is 110 - 130 for the nova model considered, compared to 110 - 440 with previous rate uncertainties. As recent type II supernova models predict ratios of 130 - 200, the 32S/33S ratio may be used to distinguish between grains of nova and supernova origin.
The fission probability of 232Pa was measured as a function of the excitation energy in order to search for hyperdeformed (HD) transmission resonances using the (d,pf) transfer reaction on a radioactive 231Pa target. The experiment was performed at t
he Tandem accelerator of the Maier-Leibnitz Laboratory (MLL) at Garching using the 231Pa(d,pf) reaction at a bombarding energy of E=12 MeV and with an energy resolution of dE=5.5 keV. Two groups of transmission resonances have been observed at excitation energies of E=5.7 and 5.9 MeV. The fine structure of the resonance group at E=5.7 MeV could be interpreted as overlapping rotational bands with a rotational parameter characteristic to a HD nuclear shape. The fission barrier parameters of 232Pa have been determined by fitting TALYS 1.2 nuclear reaction code calculations to the overall structure of the fission probability. From the average level spacing of the J=4 states, the excitation energy of the ground state of the 3rd minimum has been deduced to be E(III)=5.05 MeV.
Model predictions of the amount of the radioisotope 26Al produced in hydrogen-burning environments require reliable estimates of the thermonuclear rates for the 26gAl(p,{gamma})27Si and 26mAl(p,{gamma})27Si reactions. These rates depend upon the spec
troscopic properties of states in 27Si within about 1 MeV of the 26gAl+p threshold (Sp = 7463 keV). We have studied the 28Si(3He,{alpha})27Si reaction at 25 MeV using a high-resolution quadrupole-dipole-dipole-dipole magnetic spectrograph. For the first time with a transfer reaction, we have constrained J{pi} values for states in 27Si over Ex = 7.0 - 8.1 MeV through angular distribution measurements. Aside from a few important cases, we generally confirm the energies and spin-parity assignments reported in a recent {gamma}-ray spectroscopy study. The magnitudes of neutron spectroscopic factors determined from shell-model calculations are in reasonable agreement with our experimental values extracted using this reaction.
The discovery of naturally occurring long-lived isomeric states (t_1/2 > 10^8 yr) in the neutron-deficient isotopes 211,213,217,218Th [A. Marinov et al., Phys. Rev. C 76, 021303(R) (2007)] was reexamined using accelerator mass spectrometry (AMS). Bec
ause AMS does not suffer from molecular isobaric background in the detection system, it is an extremely sensitive technique. Despite our up to two orders of magnitude higher sensitivity we cannot confirm the discoveries of neutron-deficient thorium isotopes and provide upper limits for their abundances.
An accurate knowledge of the neutron capture cross sections of 62,63Ni is crucial since both isotopes take key positions which affect the whole reaction flow in the weak s process up to A=90. No experimental value for the 63Ni(n,gamma) cross section
exists so far, and until recently the experimental values for 62Ni(n,gamma) at stellar temperatures (kT=30 keV) ranged between 12 and 37 mb. This latter discrepancy could now be solved by two activations with following AMS using the GAMS setup at the Munich tandem accelerator which are also in perfect agreement with a recent time-of-flight measurement. The resulting (preliminary) Maxwellian cross section at kT=30 keV was determined to be <sigma>30keV = 23.4 +/- 4.6 mb. Additionally, we have measured the 64Ni(gamma,n)63Ni cross section close to threshold. Photoactivations at 13.5 MeV, 11.4 MeV and 10.3 MeV were carried out with the ELBE accelerator at Forschungszentrum Dresden-Rossendorf. A first AMS measurement of the sample activated at 13.5 MeV revealed a cross section smaller by more than a factor of 2 compared to NON-SMOKER predictions.
Analysis of presolar grains in primitive meteorites has shown isotopic ratios largely characteristic of the conditions thought to prevail in various astrophysical environments. A possible indicator for a grain of ONe nova origin is a large 33S abunda
nce: nucleosynthesis calculations predict as much as 150 times the solar abundance of 33S in the ejecta of nova explosions on massive ONe white dwarfs. This overproduction factor may, however, vary by factors of at least 0.01 - 3 because of uncertainties of several orders of magnitude in the 33S(p,gamma)34Cl reaction rate at nova peak temperatures (Tpeak ~ 0.1 - 0.4 GK). These uncertainties arise due to the lack of nuclear physics information for states within ~ 600 keV of the 33S+p threshold in 34Cl (Sp(34Cl) = 5143 keV). To better constrain this rate we have measured, for the first time, the 34S(3He,t)34Cl reaction over the region Ex(34Cl) = 4.9 - 6 MeV. We confirm previous states and find 15 new states in this energy region. New 33S(p,gamma)34Cl resonances at ER = 281(2), 301(2) and 342(2) keV may dominate this rate at relevant nova temperatures. Our results could affect predictions of sulphur isotopic ratios in nova ejecta (e.g., 32S/33S) that may be used as diagnostic tools for the nova paternity of grains.
