Second-order nonlinear effects, such as second-harmonic generation, can be strongly enhanced in nanofabricated photonic materials when both fundamental and harmonic frequencies are spatially and temporally confined. Practically designing low-volume a
nd doubly resonant nanoresonators in conventional semiconductor compounds is challenging owing to their intrinsic refractive index dispersion. In this work we review a recently developed strategy to design doubly resonant nanocavities with low mode volume and large quality factor by localized defects in a photonic crystal structure. We build on this approach by applying an evolutionary optimisation algorithm in connection with Maxwell equations solvers, showing that the proposed design recipe can be applied to any material platform. We explicitly calculate the second-harmonic generation efficiency for doubly resonant photonic crystal cavity designs in typical III-V semiconductor materials, such as GaN and AlGaAs, targeting a fundamental harmonic at telecom wavelengths, and fully accounting for the tensor nature of the respective nonlinear susceptibilities. These results may stimulate the realisation of small footprint photonic nanostructures in leading semiconductor material platforms to achieve unprecedented nonlinear efficiencies.
