Observation of Devils Staircase in the Novel Spin Valve System SrCo$_6$O$_{11}$

Using resonant soft x-ray scattering as a function of both temperature and magnetic field, we reveal a large number of almost degenerate magnetic orders in SrCo6O11. The Ising-like spins in this frustrated material in fact exhibit a so-called magnetic devils staircase. It is demonstrated how a magnetic field induces transitions between different microscopic spin configurations, which is responsible for the magnetoresistance of SrCo6O11. This material therefore constitutes a unique combination of a magnetic devils staircase and spin valve effects, yielding a novel type of magnetoresistance system.

Observation of Electronic Ferroelectric Polarization in Multiferroic YMn$_2$O$_5$

We report the observation of a magnetic polarization of the O,$2p$-states in YMn$_2$O$_5$ through the use of soft X-ray resonant scattering at the oxygen $K$-edge. Remarkably, we find that the temperature dependence of the integrated intensity of this signal closely follows the macroscopic electric polarization, and hence is proportional to the ferroelectric order parameter. This is in contrast to the temperature dependence observed at the Mn,$L_3$-edge, which reflects the Mn magnetic order parameter. First principle calculations provide a microscopic understanding of these results and show that a spin-dependent hybridization of O,$2p$- and Mn, 3d-states results in a purely electronic contribution to the ferroelectric polarization, which can exist in the absence of lattice distortions.