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59 - K. Huang 2016
Belitz-Kirkpatrick-Vojta (BKV) theory shows in excellent agreement with experiment that ferromagnetic quantum phase transitions (QPTs) in clean metals are generally first-order due to the coupling of the magnetization to electronic soft modes, in con trast to the classical analogue that is an archetypical second-order phase transition. For disordered metals BKV theory predicts that the second order nature of the QPT is restored because the electronic soft modes change their nature from ballistic to diffusive. Our low-temperature magnetization study identifies the ferromagnetic QPT in the disordered metal UCo$_{1-x}$Fe$_x$Ge as the first clear example that exhibits the associated critical exponents predicted by BKV theory.
We report the synthesis, crystal structure and characterization by means of single crystal x-ray diffraction, neutron powder diffraction, magnetic, thermal and transport measurements of the new heavy fermion compounds Ce$_{2}$MAl$_{7}$Ge$_{4}$ (M = C o, Ir, Ni, Pd). These compounds crystallize in a noncentrosymmetic tetragonal space group P={4}2$_{1}$m, consisting of layers of square nets of Ce atoms separated by Ge-Al and M-Al-Ge blocks. Ce$_{2}$CoAl$_{7}$Ge$_{4}$, Ce$_{2}$IrAl$_{7}$Ge$_{4}$ and Ce$_{2}$NiAl$_{7}$Ge$_{4}$ order magnetically behavior below $T_{M}=$ 1.8, 1.6, and 0.8 K, respectively. There is no evidence of magnetic ordering in Ce$_{2}$PdAl$_{7}$Ge$_{4}$ down to 0.4 K. The small amount of entropy released in the magnetic state of Ce$_{2}$MAl$_{7}$Ge$_{4}$ (M = Co, Ir, Ni) and the reduced specific heat jump at $T_M$ suggest a strong Kondo interaction in these materials. Ce$_{2}$PdAl$_{7}$Ge$_{4}$ shows non-Fermi liquid behavior, possibly due to the presence of a nearby quantum critical point.
YBa$_{2}$Cu$_{3}$O$_{7-{delta}}$ coated conductors (CCs) have achieved high critical current densities ($textit{J}_{c}$) that can be further increased through the introduction of additional defects using particle irradiation. However, these gains are accompanied by increases in the flux creep rate, a manifestation of competition between the different types of defects. Here, we study this competition to better understand how to design pinning landscapes that simultaneously increase $textit{J}_{c}$ and reduce creep. CCs grown by metal organic deposition show non-monotonic changes in the temperature-dependent creep rate, $textit{S}(textit{T})$. Notably, in low fields, there is a conspicuous dip to low $textit{S}$ as temperature ($textit{T}$) increases from ~20 K to ~65 K. Oxygen-, proton-, and Au-irradiation substantially increase $textit{S}$ in this temperature range. Focusing on an oxygen-irradiated CC, we investigate the contribution of different types of irradiation-induced defects to the flux creep rate. Specifically, we study $textit{S}(textit{T})$ as we tune the relative density of point defects to larger defects by annealing both an as-grown and an irradiated CC in O$_{2}$ at temperatures $textit{T}_{A}$ = 250${deg}$C to 600${deg}$C. We observe a steady decrease in $textit{S}$($textit{T}$ > 20 K) with increasing $textit{T}_{A}$, unveiling the role of pre-existing nanoparticle precipitates in creating the dip in $textit{S}(textit{T})$ and point defects and clusters in increasing $textit{S}$ at intermediate temperatures.
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