All-optical addressing and control of single solid-state based qubits allows for scalable architectures of quantum devices such as quantum networks and quantum simulators. So far, all-optical addressing of qubits was demonstrated only for color cente
rs in diamond and quantum dots. Here, we demonstrate generation of coherent dark state of a single rare earth ion in a solid, namely a cerium ion in yttrium aluminum garnet (YAG). The dark state was formed under the condition of coherent population trapping. Furthermore, high-resolution spectroscopic studies of native and implanted single Ce ions have been performed. They revealed narrow and spectrally stable optical transitions between the spin sublevels of the ground and excited optical states, indicating the feasibility of interfacing single photons with a single electron spin of a cerium ion.
We present an experimental observation of non-linear up- and down-converted optical luminescence of graphene and thin graphite subject to picosecond infrared laser pulses. We show that the excitation yields to a high density electron-hole plasma in g
raphene. It is further shown that the excited charge carries can efficiently exchange energy due to scattering in momentum space. The recombination of the resulting non-equilibrium electron-hole pairs yields to the observed white light luminescence. Due to the scattering mechanism the power dependence of the luminescence is quadratic until it saturates for higher laser power. Studying the luminescence intensity as a function of layer thickness gives further insight into its nature and provides a new tool for substrate independent thickness determination of multilayer flakes.
