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The energy barrier distribution Eb of five samples with different concentrations x of Ni nanoparticles using scaling plots from ac magnetic susceptibility data has been determined. The scaling of the imaginary part of the susceptibility Chi(nu, T) vs . Tln(t/tau_0) remains valid for all samples, which display Ni nanoparticles with similar shape and size. The mean value <E_b> increases appreciably with increasing x, or more appropriately with increasing dipolar interactions between Ni nanoparticles. We argue that such an increase in <Eb> constitutes a powerful tool for quality control in magnetic recording media technology where the dipolar interaction plays an important role.
Water ice and spin ice are important model systems in which theory can directly account for zero point entropy associated with quenched configurational disorder. Spin ice differs from water ice in the important respect that its fundamental constituen ts, the spins of the magnetic ions, can be removed through replacement with non-magnetic ions while keeping the lattice structure intact. In order to investigate the interplay of frustrated interactions and quenched disorder, we have performed systematic heat capacity measurements on spin ice materials which have been thus diluted up to 90%. Investigations of both Ho and Dy spin ices reveal that the zero point entropy depends non-monotonically on dilution and approaches the value of Rln2 in the limit of high dilution. The data are in good agreement with a generalization of Paulings theory for the entropy of ice.
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