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According to idealized models, a strong Kerr non-linearity may be used to build optical quantum gates for optical quantum information processing by inducing conditional phase shifts on quantum states. Recently, Shapiro (PRA 73, 062305 (2006)) argued that for a Kerr medium with non-instantaneous but fast response, essentially no phase shift is induced on two-single-photon input states, and thus a quantum gate build from such a medium cannot work. Here we show that a fast response Kerr medium induces some but very little phase shifts on a two-single-photon input state, and it is insufficient for high fidelity quantum computation. We point out that this is caused by the medium imparting spectral entanglement to the input photons. We further show that a way to circumvent this problem and achieve a high fidelity gate, is to engineer the dispersion properties of the medium to give a dominant spectral effect over the non-instantaneous response, in addition to satisfying a phase matching condition.
Optical $chi^{(2)}$ non-linearity can be used for parametric amplification and producing down-converted entangled photon pairs that have broad applications. It is known that weak non-linear media exhibit dispersion and produce a frequency response. I t is therefore of interest to know how spectral effects of a strong $chi^{(2)}$ crystal affect the performance. Here we model the spectral effects of the dispersion of a strong $chi^{(2)}$ crystal and illustrate how this affects its ability to perform Bell measurements and influence the performance of a quantum gates that employ such a Bell measurement. We show that a Dyson series expansion of the unitary operator is necessary in general, leading to unwanted spectral entanglement. We identify a limiting situation employing periodic poling, in which a Taylor series expansion is a good approximation and this entanglement can be removed.
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