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If magnetic frustration is most commonly known for undermining long-range order, as famously illustrated by spin liquids, the ability of matter to develop new collective mechanisms in order to fight frustration is no less fascinating, providing an av enue for the exploration and discovery of unconventional properties of matter. Here we study an ideal minimal model of such mechanisms which, incidentally, pertains to the perplexing quantum spin ice candidate Yb2Ti2O7. Specifically, we explain how thermal and quantum fluctuations, optimized by order-by-disorder selection, conspire to expand the stability region of an accidentally degenerate continuous symmetry U(1) manifold against the classical splayed ferromagnetic ground state that is displayed by the sister compound Yb2Sn2O7. The resulting competition gives rise to multiple phase transitions, in striking similitude with recent experiments on Yb2Ti2O7 [Lhotel et al., Phys. Rev. B 89 224419 (2014)]. Considering the effective Hamiltonian determined for Yb2Ti2O7, we provide, by combining a gamut of numerical techniques, compelling evidence that such multiphase competition is the long-sought missing key to understanding the intrinsic properties of this material. As a corollary, our work offers a pertinent illustration of the influence of chemical pressure in rare-earth pyrochlores.
The search for new quantum phases, especially in frustrated magnets, is central to modern condensed matter physics. One of the most promising places to look is in rare-earth pyrochlore magnets with highly-anisotropic exchange interactions, materials closely related to the spin ices Ho2Ti2O7 and Dy2Ti2O7. Here we establish a general theory of magnetic order in these materials. We find that many of their most interesting properties can be traced back to the accidental degeneracies where phases with different symmetry meet. These include the ordered ground state selection by fluctuations in Er2Ti2O7, the dimensional-reduction observed in Yb2Ti2O7, and the absence of magnetic order in Er2Sn2O7.
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