Single photons are fundamental elements for quantum information technologies such as quantum cryptography, quantum information storage and optical quantum computing. Colour centres in diamond have proven to be stable single photon sources and thus es
sential components for reliable and integrated quantum information technology. A key requirement for such applications is a large photon flux and a high efficiency. Paying tribute to various attempts to maximise the single photon flux we show that collection efficiencies of photons from colour centres can be increased with a rather simple experimental setup. To do so we spin-coated nanodiamonds containing single nitrogen-vacancy colour centres on the flat surface of a ZrO2 solid immersion lens. We found stable single photon count rates of up to 853 kcts/s at saturation under continuous wave excitation while having excess to more than 100 defect centres with count rates from 400 kcts/s to 500 kcts/s. For a blinking defect centre we found count rates up to 2.4 Mcts/s for time intervals of several ten seconds. It seems to be a general feature that very high rates are accompanied by a blinking behaviour. The overall collection efficiency of our setup of up to 4.2% is the highest yet reported for N-V defect centres in diamond. Under pulsed excitation of a stable emitter of 10 MHz, 2.2% of all pulses caused a click on the detector adding to 221 kcts/s thus opening the way towards diamond based on-demand single photon sources for quantum applications.
We present a quantum-theoretical treatment of biphoton generation in single-resonant type-II parametric down-conversion. The nonlinear medium is continuously pumped and is placed inside a cavity which is resonant for the signal field, but nonresonant
for the idler deflected by an intra-cavity polarizing beam splitter. The intensity of the classical pump is assumed to be sufficiently low in order to yield a biphoton production rate that is small compared to the cavity loss rate. Explicit expressions are derived for the rate of biphoton generation and for the biphoton wave function. The output spectra of the signal and idler field are determined, as well as the second-order signal-idler cross-correlation function which is shown to be asymmetric with respect to the time delay. Due to frequency entanglement in the signal-idler photon pair, the idler spectrum is found to reveal the longitudinal mode structure of the cavity, even though the idler field is not resonant.
