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We have investigated the (n,gamma) cross sections of p-process isotopes with the activation technique. The measurements were carried out at the Karlsruhe Van de Graaff accelerator using the 7Li(p,n)7Be source for simulating a Maxwellian neutron distr ibution of kT = 25 keV. Stellar cross section measurements are reported for the light p-process isotopes 102Pd, 120Te, 130,132Ba, and 156Dy. In a following paper the cross sections of 168Yb, 180W, 184Os, 190Pt, and 196Hg will be discussed. The data are extrapolated to p-process energies by including information from evaluated nuclear data libraries. The results are compared to standard Hauser-Feshbach models frequently used in astrophysics.
The neutron capture cross section of 14C is of relevance for several nucleosynthesis scenarios such as inhomogeneous Big Bang models, neutron induced CNO cycles, and neutrino driven wind models for the r process. The 14C(n,g) reaction is also importa nt for the validation of the Coulomb dissociation method, where the (n,g) cross section can be indirectly obtained via the time-reversed process. So far, the example of 14C is the only case with neutrons where both, direct measurement and indirect Coulomb dissociation, have been applied. Unfortunately, the interpretation is obscured by discrepancies between several experiments and theory. Therefore, we report on new direct measurements of the 14C(n,g) reaction with neutron energies ranging from 20 to 800 keV.
The stellar (n,gamma) cross section of 40Ca at kT=25 keV has been measured with a combination of the activation technique and accelerator mass spectrometry (AMS). This combination is required when direct off-line counting of the produced activity is compromised by the long half-life and/or missing gamma-ray transitions. The neutron activations were performed at the Karlsruhe Van de Graaff accelerator using the quasistellar neutron spectrum of kT=25 keV produced by the 7Li(p,n)7Be reaction. The subsequent AMS measurements were carried out at the Vienna Environmental Research Accelerator (VERA) with a 3 MV tandem accelerator. The doubly magic 40Ca is a bottle-neck isotope in incomplete silicon burning, and its neutron capture cross section determines the amount of leakage, thus impacting on the eventual production of iron group elements. Because of its high abundance, 40Ca can also play a secondary role as neutron poison for the s-process. Previous determinations of this value at stellar energies were based on time-of-flight measurements. Our method uses an independent approach, and yields for the Maxwellian-averaged cross section at kT=30 keV a value of <sigma>30 keV= 5.73+/-0.34 mb.
74 - I. Dillmann , R. Plag , M. Heil 2008
The Karlsruhe Astrophysical Database of Nucleosynthesis in Stars (KADoNiS) project is an online database for experimental cross sections relevant to the $s$ process and $p$ process. It is available under http://nuclear-astrophysics.fzk.de/kadonis and consists of two parts. Part 1 is an updated sequel to the well-known Bao et al. compilations from 1987 and 2000, which is online since April 2005. An extension of this $s$-process database to $(n,p)$ and $(n,alpha)$ cross sections at $kT$= 30 keV, as in the first version of the Bao compilation, is planned. The second part of KADoNiS is a $p$-process library, which includes all available experimental data from $(p,gamma)$, $(p,n)$, $(alpha,gamma)$, $(alpha,n)$, $(alpha,alpha)$, $(n,alpha)$ and $(gamma,n)$ reactions in or close to the respective Gamow window. Despite the great number of reactions required for a $p$-process reaction network, experimental data is still scarce and up to now restricted to stable targets. Given here is a short overview about the present status of the KADoNiS database.
We have performed $p$-process simulations with the most recent stellar $(n,gamma)$ cross sections from the Karlsruhe Astrophysical Database of Nucleosynthesis in Stars project (version v0.2, http://nuclear-astrophysics.fzk.de/kadonis). The simulation s were carried out with a parametrized supernova type II shock front model (``$gamma$ process) of a 25 solar mass star and compared to recently published results. A decrease in the normalized overproduction factor could be attributed to lower cross sections of a significant fraction of seed nuclei located in the Bi and Pb region around the $N$=126 shell closure.
The nucleosynthesis of elements beyond iron is dominated by the s and r processes. However, a small amount of stable isotopes on the proton-rich side cannot be made by neutron capture and are thought to be produced by photodisintegration reactions on existing seed nuclei in the so-called p process. So far most of the p-process reactions are not yet accessible by experimental techniques and have to be inferred from statistical Hauser-Feshbach model calculations. The parametrization of these models has to be constrained by measurements on stable proton-rich nuclei. A series of (n,$gamma$) activation measurements on p nuclei, related by detailed balance to the respective photodisintegrations, were carried out at the Karlsruhe Van de Graaff accelerator using the $^7$Li(p,n)$^7$Be source for simulating a Maxwellian neutron distribution of kT= 25 keV. We present here preliminary results of our extended measuring program in the mass range between A=74 and A=132, including first experimental (n,$gamma$) cross sections of $^{74}$Se, $^{84}$Sr, $^{120}$Te and $^{132}$Ba, and an improved value for $^{130}$Ba. In all cases we find perfect agreement with the recommended MACS predictions from the Bao et al. compilation.
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