Observation of two independent skyrmion phases in a chiral magnetic material

Magnetic materials can host skyrmions, which are topologically non-trivial spin textures. In chiral magnets with cubic lattice symmetry, all previously-observed skyrmion phases require thermal fluctuations to become thermodynamically stable in bulk materials, and therefore exist only at relatively high temperature, close to the helimagnetic transition temperature. Other stabilization mechanisms require a lowering of the cubic crystal symmetry. Here, we report the identification of a second skyrmion phase in Cu$_{2}$OSeO$_{3}$ at low temperature and in the presence of an applied magnetic field. The new skyrmion phase is thermodynamically disconnected from the well-known, nearly-isotropic, high-temperature phase, and exists, in contrast, when the external magnetic field is oriented along the $langle100rangle$ crystal axis only. Theoretical modelling provides evidence that the stabilization mechanism is given by well-known cubic anisotropy terms, and accounts for an additional observation of metastable helices tilted away from the applied field. The identification of two distinct skyrmion phases in the same material and the generic character of the underlying mechanism suggest a new avenue for the discovery, design, and manipulation of topological spin textures.

Thermodynamic evidence of a second skyrmion lattice phase and tilted conical phase in Cu$_2$0SeO$_3$

Precision measurements of the magnetization and ac susceptibility of Cu$_2$0SeO$_3$ are reported for magnetic fields along different crystallographic directions, focussing on the border between the conical and the field-polarized state for a magnetic field along the $langle 100 rangle$ axis, complemented by selected specific heat data. Clear signatures of the emergence of a second skyrmion phase and a tilted conical phase are observed, as recently identified by means of small-angle neutron scattering. The low-temperature skyrmion phase displays strongly hysteretic phase boundaries, but no dissipative effects. In contrast, the tilted conical phase is accompanied by strong dissipation and higher-harmonic contributions, while the transition fields are essentially nonhysteretic. The formation of the second skyrmion phase and tilted conical phase are found to be insensitive to a vanishing demagnetization factor. A quantitative estimate of the temperature dependence of the magnetocrystalline anisotropy may be consistently inferred from the magnetization and the upper critical field and agrees well with a stabilization of the low-temperature skyrmion phase and tilted conical state by conventional cubic magnetic anisotropies.