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151 - M. Trigo , M. Fuchs , J. Chen 2013
The macroscopic characteristics of a solid, such as its thermal, optical or transport properties are determined by the available microscopic states above its lowest energy level. These slightly higher quantum states are described by elementary excita tions and dictate the response of the system under external stimuli. The spectrum of these excitations, obtained typically from inelastic neutron and x-ray scattering, is the spatial and temporal Fourier transform of the density-density correlation function of the system, which dictates how a perturbation propagates in space and time. As frequency-domain measurements do not generally contain phase information, time-domain measurements of these fluctuations could yield a more direct method for investigating the excitations of solids and their interactions both in equilibrium and far-from equilibrium. Here we show that the diffuse scattering of femtosecond x-ray pulses produced by a free electron laser (FEL) can directly measure these density-density correlations due to lattice vibrations in the time domain. We obtain spectroscopic information of the lattice excitations with unprecedented momentum- and frequency- resolution, without resolving the energy of the outgoing photon. Correlations are created via an acoustic analog of the dynamical Casimir effect, where a femtosecond laser pulse slightly quenches the phonon frequencies, producing pairs of squeezed phonons at momenta +q and -q. These pairs of phonons manifest as macroscopic, time-dependent coherences in the displacement correlations that are then probed directly by x-ray scattering. Since the time-dependent correlations are preferentially created in regions of strong electron-phonon coupling, the time-resolved approach is natural as a spectroscopic tool of low energy collective excitations in solids, and their microscopic interactions, both in linear response and beyond.
Decays of baryon resonances in the second and the third resonance region into N pi0 pi0 are studied by photoproduction of two neutral pions off protons. Partial decay widths of N* and Delta* resonances decaying into Delta(1232) pi, N(pipi)_{S}, N(144 0)P_{11} pi, and N(1520)D_{13} pi are determined in a partial wave analysis of this data, and data from other reactions. Several partial decay widths were not known before. Interesting decay patterns are observed which are not even qualitatively reproduced by quark model calculations. In the second resonance region, decays into Delta(1232) pi dominate clearly. The N(pipi)_{S}-wave provides a significant contribution to the cross section, especially in the third resonance region. The P_{13}(1720) properties found here are at clear variance to PDG values.
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