Optical Cherenkov radiation by cascaded nonlinear interaction: an efficient source of few-cycle energetic near- to mid-IR pulses

When ultrafast noncritical cascaded second-harmonic generation of energetic femtosecond pulses occur in a bulk lithium niobate crystal optical Cherenkov waves are formed in the near- to mid-IR. Numerical simulations show that the few-cycle solitons radiate Cherenkov (dispersive) waves in the $lambda=2.2-4.5mic$ range when pumping at $lambda_1=1.2-1.8mic$. The exact phase-matching point depends on the soliton wavelength, and we show that a simple longpass filter can separate the Cherenkov waves from the solitons. The Cherenkov waves are born few-cycle with an excellent Gaussian pulse shape, and the conversion efficiency is up to 25%. Thus, optical Cherenkov waves formed with cascaded nonlinearities could become an efficient source of energetic near- to mid-IR few-cycle pulses.

Designing microstructured polymer optical fibers for cascaded quadratic soliton compression of femtosecond pulses

The dispersion of index-guiding microstructured polymer optical fibers is calculated for second-harmonic generation. The quadratic nonlinearity is assumed to come from poling of the polymer, which in this study is chosen to be the cyclic olefin copolymer Topas. We found a very large phase mismatch between the pump and the second-harmonic waves. Therefore the potential for cascaded quadratic second-harmonic generation is investigated in particular for soliton compression of fs pulses. We found that excitation of temporal solitons from cascaded quadratic nonlinearities requires an effective quadratic nonlinearity of 5 pm/V or more. This might be reduced if a polymer with a low Kerr nonlinear refractive index is used. We also found that the group-velocity mismatch could be minimized if the design parameters of the microstructured fiber are chosen so the relative hole size is large and the hole pitch is on the order of the pump wavelength. Almost all design-parameter combinations resulted in cascaded effects in the stationary regime, where efficient and clean soliton compression can be found. We therefore did not see any benefit from choosing a fiber design where the group-velocity mismatch was minimized. Instead numerical simulations showed excellent compression of $lambda=800$ nm 120 fs pulses with nJ pulse energy to few-cycle duration using a standard endlessly single-mode design with a relative hole size of 0.4.

Limits to compression with cascaded quadratic soliton compressors

We study cascaded quadratic soliton compressors and address the physical mechanisms that limit the compression. A nonlocal model is derived, and the nonlocal response is shown to have an additional oscillatory component in the nonstationary regime when the group-velocity mismatch (GVM) is strong. This inhibits efficient compression. Raman-like perturbations from the cascaded nonlinearity, competing cubic nonlinearities, higher-order dispersion, and soliton energy may also limit compression, and through realistic numerical simulations we point out when each factor becomes important. We find that it is theoretically possible to reach the single-cycle regime by compressing high-energy fs pulses for wavelengths $lambda=1.0-1.3 mu{rm m}$ in a $beta$-barium-borate crystal, and it requires that the system is in the stationary regime, where the phase mismatch is large enough to overcome the detrimental GVM effects. However, the simulations show that reaching single-cycle duration is ultimately inhibited by competing cubic nonlinearities as well as dispersive waves, that only show up when taking higher-order dispersion into account.

Scaling laws for soliton pulse compression by cascaded quadratic nonlinearities

We present a detailed study of soliton compression of ultra-short pulses based on phase-mismatched second-harmonic generation (textit{i.e.}, the cascaded quadratic nonlinearity) in bulk quadratic nonlinear media. The single-cycle propagation equations in the temporal domain including higher-order nonlinear terms are presented. The balance between the quadratic (SHG) and the cubic (Kerr) nonlinearity plays a crucial role: we define an effective soliton number -- related to the difference between the SHG and the Kerr soliton numbers -- and show that it has to be larger than unity for successful pulse compression to take place. This requires that the phase mismatch be below a critical level, which is high in a material where the quadratic nonlinearity dominates over the cubic Kerr nonlinearity. Through extensive numerical simulations we find dimensionless scaling laws, expressed through the effective soliton number, which control the behaviour of the compressed pulses. These laws hold in the stationary regime, in which group-velocity mismatch effects are small, and they are similar to the ones observed for fiber soliton compressors. The numerical simulations indicate that clean compressed pulses below two optical cycles can be achieved in a $beta$-barium borate crystal at appropriate wavelengths, even for picosecond input pulses.

Nonlocal explanation of stationary and nonstationary regimes in cascaded soliton pulse compression

We study soliton pulse compression in materials with cascaded quadratic nonlinearities, and show that the group-velocity mismatch creates two different temporally nonlocal regimes. They correspond to what is known as the stationary and nonstationary regimes. The theory accurately predicts the transition to the stationary regime, where highly efficient pulse compression is possible.