We studied alignment-to-orientation conversion caused by excited-state level crossings in a nonzero magnetic field of both atomic rubidium isotopes. Experimental measurements were performed on the transitions of the $D_2$ line of rubidium. These meas
ured signals were described by a theoretical model that takes into account all neighboring hyperfine transitions, the mixing of magnetic sublevels in an external magnetic field, the coherence properties of the exciting laser radiation, and the Doppler effect. In the experiments laser induced fluorescence (LIF) components were observed at linearly polarized excitation and their difference was taken afterwards. By observing the two oppositely circularly polarized components we were able to see structures not visible in the difference graphs, which yields deeper insight into the processes responsible for these signals. We studied how these signals are dependent on laser power density and how they are affected when the exciting laser is tuned to different hyperfine transitions. The comparison between experiment and theory was carried out fulfilling the nonlinear absorption conditions.
We have measured magneto-optical signals obtained by exciting the $D_1$ line of cesium atoms confined to an extremely thin cell (ETC), whose walls are separated by less than one micrometer, and developed an improved theoretical model to describe thes
e signals with experimental precision. The theoretical model was based on the optical Bloch equations and included all neighboring hyperfine transitions, the mixing of the magnetic sublevels in an external magnetic field, and the Doppler effect, as in previous studies. However, in order to model the extreme conditions in the ETC more realistically, the model was extended to include a unified treatment of transit relaxation and wall collisions with relaxation rates that were obtained directly from the thermal velocities of the atoms and the length scales involved. Furthermore, the interaction of the atoms with different regions of the laser beam were modeled separately to account for the varying laser beam intensity over the beam profile as well as saturation effects that become important near the center of the beam at the relatively high laser intensities used during the experiments in order to obtain measurable signals. The model described the experimentally measured signals for laser intensities for magnetic fields up to 55~G and laser intensities up to 1~W/cm$^2$ with excellent agreement.
We present the results of an experimental as well as theoretical study of nonlinear magneto-optical resonances in diatomic potassium molecules in the electronic ground state with large values of the angular momentum quantum number J~100. At zero magn
etic field, the absorption transitions are suppressed because of population trapping in the ground state due to Zeeman coherences between magnetic sublevels of this state along with depopulation pumping. The destruction of such coherences in an external magnetic field was used to study the resonances in this work. K2 molecules were formed in a glass cell filled with potassium metal at a temperature above 150C. The cell was placed in an oven and was located in a homogeneous magnetic field B, which was scanned from zero to 0.7 T. Q-type and R-type transitions were excited with a tunable, single-mode diode laser with central wavelength of 660 nm. Well pronounced nonlinear Hanle effect signals were observed in the intensities of the linearly polarized components of the laser-induced fluorescence (LIF) detected in the direction parallel to the (B)-field with polarization vectors parallel (I_par) and perpendicular (I_per) to the polarization vector of the exciting laser radiation, which was orthogonal to (B). The intensities of the LIF components were detected for different experimental parameters, such as laser power density and vapor temperature, in order to compare them with numerical simulations that were based on the optical Bloch equations for the density matrix. We report good agreement of our measurements with numerical simulations. Narrow, subnatural line width dark resonances in I_per(B) were detected and explained.
Nonlinear magneto-optical resonances have been measured in an extremely thin cell (ETC) for the D1 transition of rubidium in an atomic vapor of natural isotopic composition. All hyperfine transitions of both isotopes have been studied for a wide rang
e of laser power densities, laser detunings, and ETC wall separations. Dark resonances in the laser induced fluorescence (LIF) were observed as expected when the ground state total angular momentum F_g was greater than or equal to the excited state total angular momentum F_e. Unlike the case of ordinary cells, the width and contrast of dark resonances formed in the ETC dramatically depended on the detuning of the laser from the exact atomic transition. A theoretical model based on the optical Bloch equations was applied to calculate the shapes of the resonance curves. The model averaged over the contributions from different atomic velocity groups, considered all neighboring hyperfine transitions, took into account the splitting and mixing of magnetic sublevels in an external magnetic field, and included a detailed treatment of the coherence properties of the laser radiation. Such a theoretical approach had successfully described nonlinear magneto-optical resonances in ordinary vapor cells. Although the values of certain model parameters in the ETC differed significantly from the case of ordinary cells, the same physical processes were used to model both cases. However, to describe the resonances in the ETC, key parameters such as the transit relaxation rate and Doppler width had to be modified in accordance with the ETCs unique features. Agreement between the measured and calculated resonance curves was satisfactory for the ETC, though not as good as in the case of ordinary cells.
Experimental signals of non-linear magneto-optical resonances at D1 excitation of natural rubidium in a vapor cell have been obtained and described with experimental accuracy by a detailed theoretical model based on the optical Bloch equations. The D
1 transition of rubidium is a challenging system to analyze theoretically because it contains transitions that are only partially resolved under Doppler broadening. The theoretical model took into account all nearby transitions, the coherence properties of the exciting laser radiation, and the mixing of magnetic sublevels in an external magnetic field and also included averaging over the Doppler profile. Great care was taken to obtain accurate experimental signals and avoid systematic errors. The experimental signals were reproduced very well at each hyperfine transition and over a wide range of laser power densities, beam diameters, and laser detunings from the exact transition frequency. The bright resonance expected at the F_g=1 --> F_e=2 transition of Rb-87 has been observed. A bright resonance was observed at the F_g=2 --> F_e=3 transition of Rb-85, but displaced from the exact position of the transition due to the influence of the nearby F_g=2 --> F_e=2 transition, which is a dark resonance whose contrast is almost two orders of magnitude larger than the contrast of the bright resonance at the F_g=2 --> F_e=3 transition. Even in this very delicate situation, the theoretical model described in detail the experimental signals at different laser detunings.
Experimental and theoretical studies are presented related to the ground-state magneto-optical resonance prepared in Cesium vapour confined in an Extremely Thin Cell (ETC, with thickness equal to the wavelength of the irradiating light). It is shown
that the utilization of the ETC allows one to examine the formation of a magneto-optical resonance on the individual hyperfine transitions, thus distinguishing processes resulting in dark (reduced absorption) or bright (enhanced absorption) resonance formation. We report on an experimental evidence of the bright magneto-optical resonance sign reversal in Cs atoms confined in the ETC. A theoretical model is proposed based on the optical Bloch equations that involves the elastic interaction processes of atoms in the ETC with its walls resulting in depolarization of the Cs excited state which is polarized by the exciting radiation. This depolarization leads to the sign reversal of the bright resonance. Using the proposed model, the magneto-optical resonance amplitude and width as a function of laser power are calculated and compared with the experimental ones. The numerical results are in good agreement with the experiment.
