We investigate the coherent manipulation of interacting Rydberg atoms placed inside a high-finesse optical cavity for the deterministic preparation of strongly coupled light-matter systems. We consider a four-level diamond scheme with one common Rydb
erg level for N interacting atoms. One side of the diamond is used to excite the atoms into a collective `superatom Rydberg state using either {pi}-pulses or stimulated Raman adiabatic passage (STIRAP) pulses. The upper transition on the other side of the diamond is used to transfer the collective state to one that is coupled to a field mode of an optical cavity. Due to the strong interaction between the atoms in the Rydberg level, the Rydberg blockade mechanism plays a key role in the deterministic quantum state synthesis of the atoms in the cavity. We use numerical simulation to show that non-classical states of light can be generated and that the state that is coupled to the cavity field is a collective one. We also investigate how different decay mechanisms affect this interacting many-body system. We also analyze our system in the case of two Rydberg excitations within the blockade volume. The simulations are carried out with parameters corresponding to realizable high-finesse optical cavities and alkali atoms like rubidium.
