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We report measurements and theoretical analysis of resonant spin tunneling in randomly oriented nanospheres of a molecular magnet. Amorphous nanospheres of Mn$_{12}$ acetate have been fabricated and characterized by chemical, infrared, TEM, X-ray, an d magnetic methods. Magnetic measurements have revealed sharp tunneling peaks in the field derivative of the magnetization that occur at the typical resonant field values for Mn$_{12}$ acetate. Theoretical analysis is provided that explains these observations. We argue that resonant spin tunneling in a molecular magnet can be established in a powder sample, without the need for a single crystal and without aligning the easy magnetization axes of the molecules. This is confirmed by re-analyzing the old data on a powdered sample of non-oriented micron-size crystals of Mn$_{12}$ acetate. Our findings can greatly simplify the selection of candidates for quantum spin tunneling among newly synthesized molecular magnets.
We have studied Josephson tunneling through a circularly polarized micron or submicron-size disk of a soft ferromagnetic material. Such a disk contains a vortex that exhibits rich classical dynamics and has recently been proposed as a tool to study q uantum dynamics of the nanoscale vortex core. The change in the Josephson current that is related to a tiny displacement of the vortex core has been computed analytically and plotted numerically for permalloy disks used in experiments. It is shown that a Josephson junction with a magnetic disk in the vortex state can be an interesting physical system that may be used to measure the nanoscale motion of the magnetic vortex.
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