We demonstrate experimentally that spontaneous parametric down-conversion in an AlGaAs semiconductor Bragg reflection waveguide can make for paired photons highly entangled in the polarization degree of freedom at the telecommunication wavelength of
1550 nm. The pairs of photons show visibility higher than 90% in several polarization bases and violate a Clauser-Horne-Shimony-Holt Bell-like inequality by more than 3 standard deviations. This represents a significant step toward the realization of efficient and versatile self pumped sources of entangled photon pairs on-chip.
It is controversial what is the true role of entanglement in two-photon virtual-state spectroscopy [Saleh et al, Phys. Rev. Lett. 80, 3483, 1998], a two-photon absorption spectroscopic technique that can retrieve information about the energy level st
ructure of an atom or a molecule. The consideration of closely related techniques, such as multidimensional pump-probe spectroscopy [Roslyak et al, Phys. Rev. A 79, 063409, 2009], might suggest that spectroscopic information retrieved in the two-photon absorption process is the same regardless of the classical or quantum nature of the light source. Here, we solve this debate by making use of a full quantum formalism to show that the ability to obtain information about the energy level structure of a medium requires the existence of temporal (frequency) correlations between the absorbed photons. Moreover, we show that these correlations are not the only requisite for retrieving such information. In fact, it is a combination of both, the presence of frequency correlations and its specific spectral shape, which makes the realization of two-photon virtual-state spectroscopy possible. This result helps clarifying the discussion whether entanglement is needed or not, and also, to specify the type of two-photon source that needs to be used in order to experimentally perform the two-photon virtual-state spectroscopy technique.
