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We report on the real space profile of spin polarons in the quasi two-dimensional frustrated dimer spin system SrCu2(BO3)2 doped with 0.16% of Zn. The 11B nuclear magnetic resonance spectrum exhibits 15 additional boron sites near non-magnetic Zn imp urities. With the help of exact diagonalizations of finite clusters, we have deduced from the boron spectrum the distribution of local magnetizations at the Cu sites with fine spatial resolution, providing direct evidence for an extended spin polaron. The results are confronted with those of other experiments performed on doped and undoped samples of SrCu2(BO3)2.
266 - H. Kobayashi , T. Nagao , M. Itou 2009
Two-dimensional spin-uncompensated momentum density distributions, $rho_{rm s}^{2D}({bf p})$s, were reconstructed in magnetite at 12K and 300K from several measured directional magnetic Compton profiles. Mechanical de-twinning was used to overcome se vere twinning in the single crystal sample below the Verwey transition. The reconstructed $rho_{rm s}^{2D}({bf p})$ in the first Brillouin zone changes from being negative at 300 K to positive at 12 K. This result provides the first clear evidence that electrons with low momenta in the minority spin bands in magnetite are localized below the Verwey transition temperature.
High degree of preservation of spin states during energy relaxation processes mediated by optical phonons is demonstrated in a single quantum dot. Optical-phonon resonance and relevant suppression of spin relaxation are clearly identified as dip stru ctures in photoluminescence excitation spectra probed by the positive trion emission. The absence of continuum states makes this observation possible under the cross-circularly polarized detection with respect to a circularly polarized pumping. Consequently, distinguishably high degree of circular polarization up to ~0.85 is achieved without applying external magnetic field at the optical-phonon resonance. Rate equation analysis reveals that the spin-flip probability during energy relaxation is restricted to less than 7.5%. It is also indicated that the spin flip time of the positive trion ground state is extended by more than 3 times compared with that of neutral exciton ground state. This corresponds to the spin flip time longer than 11 ns for the positive trion ground state. The influence of nuclear polarization to the present measurements is also discussed.
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